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Record W2467079137 · doi:10.1039/c6sm01238h

Chiral oily streaks in a smectic-A liquid crystal

2016· article· en· W2467079137 on OpenAlexaff
Ian R. Nemitz, Andrew J. Ferris, Emmanuelle Lacaze, Charles Rosenblatt

Bibliographic record

VenueSoft Matter · 2016
Typearticle
Languageen
FieldMaterials Science
TopicLiquid Crystal Research Advancements
Canadian institutionsCanadian Nautical Research Society
FundersDivision of Materials ResearchCentre National de la Recherche ScientifiqueAgence Nationale de la RechercheNational Science Foundation
KeywordsLiquid crystalMaterials scienceDopantSubstrate (aquarium)PerpendicularPolarizerRotation (mathematics)OpticsCondensed matter physicsPolarized light microscopyPhase (matter)Homeotropic alignmentFréedericksz transitionDopingElectric fieldPlanarCrystallographyBirefringenceChemistryOptoelectronicsGeometryPhysics

Abstract

fetched live from OpenAlex

The liquid crystal octylcyanobiphenyl (8CB) was doped with the chiral agent CB15 and spin-coated onto a substrate treated for planar alignment of the director, resulting in a film of thickness several hundred nm in the smectic-A phase. In both doped and undoped samples, the competing boundary conditions - planar alignment at the substrate and vertical alignment at the free surface - cause the liquid crystal to break into a series of flattened hemicylinders to satisfy the boundary conditions. When viewed under an optical microscope with crossed polarizers, this structure results in a series of dark and light stripes ("oily streaks") of period ∼1 μm. In the absence of chiral dopant the stripes run perpendicular to the substrate's easy axis. However, when doped with chiral CB15 at concentrations up to c = 4 wt%, the stripe orientation rotates by a temperature-dependent angle φ with respect to the c = 0 stripe orientation, where φ increases monotonically with c. φ is largest just below the nematic - smectic-A transition temperature TNA and decreases with decreasing temperature. As the temperature is lowered, φ relaxes to a steady-state orientation close to zero within ∼1 °C of TNA. We suggest that the rotation phenomenon is a manifestation of the surface electroclinic effect: The rotation is due to the weak smectic order parameter and resulting large director tilt susceptibility with respect to the smectic layer normal near TNA, in conjunction with an effective surface electric field due to polar interactions between the liquid crystal and substrate.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.034
Threshold uncertainty score0.995

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0070.006

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.276
Teacher spread0.262 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2016
Admission routes1
Has abstractyes

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