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Record W2473202533 · doi:10.1139/cjp-2016-0252

Experimental and theoretical investigation of molecular structure, vibrational analysis, chemical reactivity, electrostatic potential of benzyl methacrylate monomer and homopolymer

2016· article· en· W2473202533 on OpenAlexvenueno aff
Feride Akman

Bibliographic record

VenueCanadian Journal of Physics · 2016
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Synthesis and Characterization
Canadian institutionsnot available
FundersBitlis Eren Üniversitesi
KeywordsMonomerBasis setMolecular orbitalMulliken population analysisComputational chemistryDensity functional theoryPolymerMethacrylateMolecular geometryMoleculePhysical chemistryMaterials scienceChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Until now, a number of new polymers have been discovered with the aid of experimental and computational molecular approaches and indicated to have potential applications. All the computational molecular approaches provide information helpful to further study. So, monomer and homopolymer of benzyl methacrylate (BzMA), which is a popular methacrylate ester monomer, were synthesized and investigated based on density functional theory (DFT) and Hartree–Fock (HF) methods. The monomer and homopolymer were characterized by FTIR, 1H, and 13C NMR techniques. The molecular geometry, geometrical parameters, Mulliken atomic charges, and vibrational frequencies of BzMA monomer and homopolymer (in dimer form) were calculated by using the DFT and HF methods with 6-31G (d, p) as basis set. The molecular electrostatic potential maps and molecular orbitals properties of monomer and homopolymer were calculated using the 6-31G (d, p) basis set of theories. Besides, 1H and 13C chemical shifts were calculated by the gauge–including atomic orbital approach. The results demonstrated that the theoretical values were in good agreement with the experimental values. The calculated data are important to providing insight into molecular analysis and may be used in technological applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.017

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0050.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.201
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations30
Published2016
Admission routes1
Has abstractyes

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