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Record W2475690610 · doi:10.1021/bk-2010-1043.ch024

Sustained Development in Baeyer-Villiger Biooxidation Technology

2010· book-chapter· en· W2475690610 on OpenAlexaff
Peter C. K. Lau, Hannes Leisch, Brahm J. Yachnin, I.A. Mirza, Albert M. Berghuis, Hiroaki Iwaki, Yoshie Hasegawa

Bibliographic record

VenueACS symposium series · 2010
Typebook-chapter
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicSteroid Chemistry and Biochemistry
Canadian institutionsMcGill UniversityBiotechnology Research InstituteNational Research Council Canada
Fundersnot available
KeywordsBiotransformationMonooxygenaseCofactorEnantioselective synthesisChemistryBiocatalysisCyclohexanoneStereochemistryBiochemistryCatalysisEnzymeCytochrome P450Reaction mechanism

Abstract

fetched live from OpenAlex

From the first crystal structures of a prototypical cyclohexanone monooxygenase (CHMO) complexed with both FAD and NADP+ cofactors to whole genome mining of new microbial Baeyer-Villiger monooxygenases (BVMOs), this review highlights the recent progress in Baeyer-Villiger biooxidation technology. Protein engineering of BVMOs as enantioselective enzymes in asymmetric catalysis to accommodate new substrates is an active pursuit. Cofactor recycling appears to no longer be an issue, and we have gained a greater understanding of whole-cell biotransformation dynamics and limitations, leading us towards industrial scale realization. In terms of substrate profiling, new naturally-occurring substrates have been found in addition to a seeming rebirth of interest in BVMO-mediated oxidation of steroids.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Research integrity
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.325
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.001
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0020.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.203
Teacher spread0.197 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2010
Admission routes1
Has abstractyes

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