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Record W2511300684 · doi:10.15278/isms.2016.wj09

SPECTROSCOPY OF THE X1Σ+, A1Π and B1Σ+ ELECTRONIC STATES OF MgS

2016· article· en· W2511300684 on OpenAlexaff
D. W. Tokaryk, C. Linton, A. G. Adam, Nicholas S. Caron

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsUniversity of New Brunswick
Fundersnot available
KeywordsDiatomic moleculeIsotopologueLaser-induced fluorescenceSpectral lineRydberg stateGround stateAbsorption spectroscopyRotational spectroscopyAtomic physicsSpectroscopyFluorescenceAtomic electron transitionLaser ablationLaserMaterials scienceAnalytical Chemistry (journal)Rydberg formulaChemistryMoleculePhysicsOpticsIonIonization

Abstract

fetched live from OpenAlex

The spectra of some astrophysical sources contain signatures from molecules containing magnesium or sulphur atoms. Therefore, we have extended previous studies of the diatomic molecule \\chem{MgS}, which is a possible candidate for astrophysical detection. Microwave spectra of X$^1\\Sigma^+$ , the ground electronic state, were reported in 1989\\footnote{S. Takano, S. Yamamoto and S. Saito, Chem. Phys. Lett. \\textbf{159}, 563-566 (1989).} and 1997\\footnote{K. A. Walker and M. C. L. Gerry, J. Mol. Spectrosc \\textbf{182}, 178-183 (1997).}, and the B$^1\\Sigma^+$--X$^1\\Sigma^+$ electronic absorption spectrum in the blue was last studied in 1970\\footnote{M. Marcano and R. F. Barrow, Trans. Faraday Soc. \\textbf{66}, 2936-2938 (1970).}. We have investigated the B$^1\\Sigma^+$--X$^1\\Sigma^+$ 0-0 spectrum of \\chem{MgS} at high resolution under jet-cooled conditions in a laser-ablation molecular source, and have obtained laser-induced fluorescence spectra from four isotopologues. Dispersed fluorescence from this source identified the low-lying A$^1\\Pi$ state near 4520 \\wn. We also created \\chem{MgS} in a Broida oven, with the help of a stream of activated nitrogen, and took rotationally resolved dispersed fluorescence spectra of the B$^1\\Sigma^+$--A$^1\\Pi$ transition with a grating spectrometer by laser excitation of individual rotational levels of the B$^1\\Sigma^+$ state via the B$^1\\Sigma^+$--X$^1\\Sigma^+$ transition. These spectra provide a first observation and analysis of the A$^1\\Pi$ state.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.022
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.218
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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