MétaCan
Menu
Back to cohort
Record W2513727561 · doi:10.1021/acs.iecr.5b03929

Determination of Diffusion Coefficient for Alkane Solvent–CO<sub>2</sub> Mixtures in Heavy Oil with Consideration of Swelling Effect

2016· article· en· W2513727561 on OpenAlexafffund
Sixu Zheng, Huazhou Li, Huijuan Sun, Daoyong Yang

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2016
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsUniversity of Regina
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsSwellingDiffusionSolventChemistryAlkaneThermodynamicsPartition coefficientDissolutionMass transferEffective diffusion coefficientHydrocarbonVolume (thermodynamics)Mass transfer coefficientPhase (matter)Analytical Chemistry (journal)Materials scienceChromatographyOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

A generalized methodology has been developed and successfully applied to determine diffusion coefficient of alkane solvent–CO 2 –heavy oil systems with consideration of swelling effect. Theoretically, a one-dimensional and one-way mass transfer model incorporating the volume translated Peng–Robinson equation of state (PR EOS) has been developed to describe the mass transfer from alkane solvent–CO 2 mixture to heavy oil, which accounts for the oil swelling effect resulted from gas dissolution. The heavy oil sample has been characterized as three pseudocomponents, while the binary interaction parameter (BIP) correlations are tuned with the experimentally measured saturation pressures. Both apparent diffusion coefficients for gas mixtures and individual diffusion coefficient of each component of a mixture are determined once the discrepancy between the measured and calculated dynamic swelling factors of heavy oil has been minimized. The volume translated PR EOS with the three characterized pseudocomponents and the tuned BIP correlations is able to accurately predict the phase behavior of alkane solvent–CO 2 –heavy oil systems. Compared to the apparent diffusion coefficient, better agreements between the measured and calculated dynamic swelling factors have been obtained by use of the individual diffusion coefficients. Addition of C 3 H 8 into CO 2 stream is found to not only diffuse faster into heavy oil than CO 2 but also contribute to a larger degree of oil swelling, leading to a faster and enhanced swelling effect of C 3 H 8 –CO 2 –heavy oil system in comparison with the CO 2 –heavy oil system.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.284
Teacher spread0.256 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations95
Published2016
Admission routes2
Has abstractyes

Explore more

Same venueIndustrial & Engineering Chemistry ResearchSame topicPhase Equilibria and ThermodynamicsFrench-language works237,207