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Record W2515492736 · doi:10.15278/isms.2016.mi04

STRUCTURAL ANALYSIS OF 2-FLUOROPHENOL AND 3-FLUOROPHENOL USING FTMW SPECTROSCOPY

2016· article· en· W2515492736 on OpenAlexaff
Aimee Bell, Jennifer van Wijngaarden, J.V.L. Singer, Omar Mahassneh

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldChemistry
TopicInorganic and Organometallic Chemistry
Canadian institutionsUniversity of Manitoba
Fundersnot available
KeywordsComputer science

Abstract

fetched live from OpenAlex

The ground states of 2-fluorophenol (2-FPh) and 3-fluorophenol (3-FPh) were studied using Fourier transform microwave (FTMW) techniques to record their rotational spectra in the range of 6 to 26 GHz. Two planar conformers of similar energy were observed for 3-FPh (cis, trans) while only the lowest energy conformer (cis) of 2-FPh was observed due to the stabilizing effect of an intramolecular interaction between fluorine and OH. Rotational constants derived from spectra of the $^{13}$C analogs, observed in natural abundance, were used to calculate the substitution (r$_{s}$) and effective ground state (r$_{0}$) parameters for cis-2-FPh and trans-3-FPh in order to study the effect of fluorination at sites along the benzene backbone. Geometry optimization at the MP2/6-311++G(2d,2p) level was used obtain the equilibrium (r$_{e}$) structures for comparison. Furthermore, natural bond order (NBO) calculations provided supporting information of a OH•••F interaction in cis-2-FPh.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.023
Threshold uncertainty score0.978

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0230.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.236
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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