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Record W2517838794 · doi:10.1021/acs.iecr.5b03003

Synthesis and Characterization of Co/C and Fe/C Nanocatalysts for Fischer–Tropsch Synthesis: A Comparative Study Using a Fixed-Bed Reactor

2015· article· en· W2517838794 on OpenAlexaff
James Aluha, Philip Boahene, Ajay K. Dalai, Yongfeng Hu, Kossi E. Béré, Nadi Braidy, Nicolas Abatzoglou

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2015
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsCanadian Light Source (Canada)University of SaskatchewanUniversité de Sherbrooke
Fundersnot available
KeywordsFischer–Tropsch processCatalysisSpace velocityNanomaterial-based catalystSyngasChemical engineeringMaterials scienceCoprecipitationChemistryBar (unit)Inorganic chemistryOrganic chemistrySelectivity

Abstract

fetched live from OpenAlex

Production of Fischer–Tropsch catalysts is challenging because it involves controlling and optimizing multiple parameters in numerous technical steps. Here, we present C-supported nanometric Fe and Co catalysts synthesized by plasma spraying, a method that contracts catalyst production into a single step, in contrast to traditional multistep catalyst production by precipitation or impregnation. The catalysts were reduced in situ and then tested for Fischer–Tropsch synthesis in a gas–solid fixed-bed reactor at 230 °C and 30-bar pressure for 24 h. The performance of plasma-synthesized catalysts was superior at a gas hourly space velocity of 6,000 mL·g cat –1 ·h –1, with Fe/C catalysts showing about 30% CO conversion per pass while Co/C catalysts yielded about 20% CO conversion. Identical C-supported Co and Fe catalysts prepared by impregnation or precipitation gave CO conversions of about 7% under similar reaction conditions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.192
GPT teacher head0.370
Teacher spread0.178 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations28
Published2015
Admission routes1
Has abstractyes

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