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Record W2520392447 · doi:10.1021/acs.inorgchem.6b01467

AlFe<sub>2–<i>x</i></sub>Co<sub><i>x</i></sub>B<sub>2</sub> (<i>x</i> = 0–0.30): <i>T</i><sub>C</sub> Tuning through Co Substitution for a Promising Magnetocaloric Material Realized by Spark Plasma Sintering

2016· article· en· W2520392447 on OpenAlexaff
Sarah Hirt, Fang Yuan, Yurij Mozharivskyj, Harald Hillebrecht

Bibliographic record

VenueInorganic Chemistry · 2016
Typearticle
Languageen
FieldMaterials Science
TopicMXene and MAX Phase Materials
Canadian institutionsMcMaster University
Fundersnot available
KeywordsChemistryFerromagnetismParamagnetismMagnetic refrigerationSpark plasma sinteringCrystallographyMagnetizationRietveld refinementCobaltAnalytical Chemistry (journal)Curie temperatureArc meltingPowder diffractionCrystal structureCondensed matter physicsInorganic chemistryMagnetic field

Abstract

fetched live from OpenAlex

AlFe 2 B 2 and AlFe 2– x Co x B 2 ( x = 0–0.30) were synthesized from the elements in three different ways. The samples were characterized by powder X-ray diffraction, Rietveld refinements, energy-dispersive X-ray spectroscopy, and magnetic measurements. Using Al flux the formation of AlFe 2 B 2 single crystals is preferred. Arc melting enables the substitution of ∼6% Co. This substitution of Fe by Co decreases the Curie temperature T C from 290 to 240 K. The highest Co substitution up to 15% is achieved by spark plasma sintering (SPS). T C is reduced to 205 K. In all cases an excess of Al is necessary to avoid the formation of ferromagnetic FeB. Al 13 Fe 4– x Co x is the common byproduct. T C and the cobalt content are linearly correlated. The transition paramagnetic–ferromagnetic remains sharp for all examples. The magnetic entropy change of the Co-containing samples is comparable to AlFe 2 B 2 . SPS synthesis yields, in short reaction times, a homogeneous and dense material with small amounts of paramagnetic Al 13 Fe 4–x Co x as an impurity, which can serve as sinter additive. These properties make AlFe 2– x Co x B 2 a promising magnetocaloric material for applications between room temperature and 200 K.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.239
Teacher spread0.225 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations67
Published2016
Admission routes1
Has abstractyes

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