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Record W2524424633 · doi:10.1002/cnma.201600251

Photocatalytic Properties of All Four Polymorphs of Nanostructured Iron Oxyhydroxides

2016· article· en· W2524424633 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueChemNanoMat · 2016
Typearticle
Languageen
FieldEnergy
TopicIron oxide chemistry and applications
Canadian institutionsYork UniversityUniversity of Toronto
Fundersnot available
KeywordsAkaganéiteLepidocrociteGoethitePhotocatalysisMaterials scienceMethylene blueVisible spectrumNanoparticleChemical engineeringNuclear chemistryChemistryNanotechnologyPhysical chemistryOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

Abstract Four different polymorphs of nanostructured iron oxyhydroxides, namely; goethite (α‐FeOOH), akaganeite (β‐FeOOH), lepidocrocite (γ‐FeOOH), and feroxyhyte (δ‐FeOOH) were synthesized and fully characterized by X‐ray diffraction, electron microscopy, UV/Visible spectrophotometry, Brunauer–Emmett–Teller (BET) measurements, and X‐ray photoemission spectroscopy. The relationship between these iron oxyhydroxide polymorphs and their photocatalytic properties was explored by examining the extent of methylene blue (MB) degradation by each polymorph under visible‐light irradiation. Feroxyhyte exhibited the best photocatalytic properties and degraded 85 % of the MB dye in five hours. In comparison, goethite, akaganeite, and lepidocrocite degraded only 40 %, 35 %, and 30 % of the MB in five hours, respectively. To understand this trend, the surface area, particle size and shape, and electronic band properties were systematically studied and discussed. It was found that the rate of MB degradation relates mainly to the surface area of the FeOOH polymorphs more than any other factor. This is the first report of a comparative study of the physical, electronic, and photocatalytic properties of all four polymorphs of nanostructured iron oxyhydroxides.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.423

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.214
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it