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Record W2530054608 · doi:10.33915/etd.7316

Solid state formation of calcium carbide

2014· dissertation· en· W2530054608 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

Venuenot available
Typedissertation
Languageen
FieldChemistry
TopicMulticomponent Synthesis of Heterocycles
Canadian institutionsnot available
FundersCanada Excellence Research Chairs, Government of CanadaU.S. Department of Energy
KeywordsAcetyleneCalcium carbideMaterials scienceCalcium oxideAnalytical Chemistry (journal)CarbideCarbon fibersX-ray photoelectron spectroscopyRaw materialChemical engineeringChemistryMetallurgyOrganic chemistryComposite materialComposite number

Abstract

fetched live from OpenAlex

Acetylene is known as an essential chemical building block with increasing prominent applications as a raw material in the production of important organic compounds. An indirect method used to synthesize acetylene is through the decomposition of CaC2 in the presence of water. The current work investigated a process for the synthesis of calcium carbide via a solid-state reaction route and the general kinetics of the reaction was characterized. The calcium carbide was synthesized by conventional and microwave heating (6 kW, 2.45GHz) of micron-sized calcium oxide and carbon powders in argon. The temperature range for these reactions was between 1000--1800°C. The work succeeded in preparing CaC2 within several minutes using microwave heating. A well-crystallized product was obtained with purities as high as 90% CaC2. Three different phase were identified during the reactions depending upon the temperature regime; CaC2 II (at 1600°C), CaC2 II & III (at 1650°C) and CaC2 I, II & III (at 1700°C) were identified using a x-ray diffraction phase identification technique. The apparent activation energy calculated was found to be approximately 125.66 kJ·mol-1.;In addition to variation in reaction temperature, uniaxial pellet compaction load, reaction times, sample mass and heating rates were also varied. The influence of solid particle surface contact, carbon source reactivity and mold configuration were included in this investigation. The effects of the processing techniques and variables on the final density, microstructural properties and percent purity of the resulting products were characterized using the gas chromatograph, X-ray photoelectron spectroscopy and X-ray diffraction techniques.;Finally, the calcium carbide synthesized via microwave heating yielded 80% more carbide formed compared to conventionally processed carbide at 1600°C. The reaction kinetics was increased for all temperatures using the same feed amount. The density and degree of purity of the products were affected by reaction temperature and exposure time, starting particle size of the reactants and the dimension of the sample container.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.062
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.305
Teacher spread0.284 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Quick stats

Citations1
Published2014
Admission routes1
Has abstractyes

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