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Record W2531154020 · doi:10.1021/acs.iecr.6b03018

Artificial Neural Networks for Accurate Prediction of Physical Properties of Aqueous Quaternary Systems of Carbon Dioxide (CO<sub>2</sub>)-Loaded 4-(Diethylamino)-2-butanol and Methyldiethanolamine Blended with Monoethanolamine

2016· article· en· W2531154020 on OpenAlexafffund
Fatemeh Pouryousefi, Raphael Idem, Teeradet Supap, Paitoon Tontiwachwuthikul

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2016
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsUniversity of Regina
FundersNatural Sciences and Engineering Research Council of CanadaCanada Foundation for InnovationFaculty of Graduate Studies and Research, University of Regina
KeywordsThermal diffusivityAmine gas treatingCarbon dioxideAqueous solutionChemistryCorrelation coefficientViscosityAlkanolamineMaterials scienceAnalytical Chemistry (journal)ThermodynamicsChromatographyOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Physical and heat transport properties such as density, viscosity, refractive index, heat capacity, thermal conductivity, and thermal diffusivity of aqueous carbon dioxide (CO 2 )-loaded and unloaded 4-(diethyl amino)-2-buthanol (DEAB) and methyldiethanolamine (MDEA) as single amines and each blended with a primary amine (MEA) were measured at different ranges of temperature (25–60 °C), amine concentrations (0.5–2 M for tertiary amine and 5 M for primary amine), and CO 2 loading (0–0.6 mol/mol amine). Results showed an increasing trend of CO 2 loading on density, viscosity, and refractive index and a decreasing trend on the heat transport properties. Two artificial neural network techniques, back propagation neural network (BPNN) and radial basis neural network (RBFNN) as well as some well-known semi-empirical correlations from literature, were applied to correlate and predict these physical properties for two quaternary systems: MEA+DEAB+water+CO 2 and MEA+MDEA+water+CO 2 . Results from the correlation showed that artificial neural network techniques gave the least deviation for the prediction of all physical properties of both amine systems with less than 1% AAD. The correlation coefficient between the experimental and predicted values in terms of R 2 value was in the range of 0.98–0.99.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.343
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.056
GPT teacher head0.265
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2016
Admission routes2
Has abstractyes

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