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Characterization of Heavy Distillation Cuts Using Fourier Transform Infrared Spectrometry: Proof of Concept

2016· article· en· W2552370257 on OpenAlexaff
M. C. Sánchez-Lemus, F. F. Schoeggl, Shawn D. Taylor, Simon Ivar Andersen, Mmilili M. Mapolelo, M. Sharath Chandra, Harvey W. Yarranton

Bibliographic record

VenueEnergy & Fuels · 2016
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsSchlumberger (Canada)University of Calgary
Fundersnot available
KeywordsFourier transform infrared spectroscopyDistillationAnalytical Chemistry (journal)FractionationChemistryInfraredFourier transformVacuum distillationPhysical propertyMass fractionMass spectrometryInfrared spectroscopyFraction (chemistry)Spectral lineChromatographyOrganic chemistryOpticsPhysics

Abstract

fetched live from OpenAlex

Fourier transform infrared spectrometry (FTIR) spectra were measured for 16 distillation cuts obtained from two bitumens using a deep vacuum fractionation apparatus. Three regions of the spectra were deconvoluted into peaks each associated with a known type of vibration: (1) aliphatic C–H stretching in the 2800–3000 cm –1 region, (2) aliphatic C–H scissoring/symmetric deformation in the 1350–1400 cm –1 region, and (3) aromatic C–H out-of-plane bending in the 680–900 cm –1 region. The distribution of chemical structures in the oils were assessed, and preliminary correlations were identified between measured physical properties (density, atomic H/C ratio, and molecular weight) and the quantified peak areas obtained from the FTIR spectra. A preliminary method was proposed to generate physical property distribution data for crude oils based on distillation and FTIR data. The method predicted the density, atomic H/C ratio, and molecular weight of the distillation cuts, with average deviations less than 0.8, 1.4, and 16%, respectively. Note that the method was tested on the same cuts used to generate the correlations because there were insufficient data for an independent test.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.227
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2016
Admission routes1
Has abstractyes

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