Competing orders and topology in the global phase diagram of pyrochlore iridates
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Bibliographic record
Abstract
Strong electronic interactions and spin-orbit coupling can be conducive for realizing novel broken symmetry phases supporting quasiparticles with nontrivial band topology. 227 pyrochlore iridates provide a suitable material platform for studying such emergent phenomena where both topology and competing orders play important roles. In contrast to the most members of this material class, which are thought to display ``all-in--all-out'' (AIAO) type magnetically ordered low-temperature insulating ground states, ${\mathrm{Pr}}_{2}{\mathrm{Ir}}_{2}{\mathrm{O}}_{7}$ remains metallic while exhibiting ``spin-ice'' (SI) correlations at low temperatures. Additionally, this is the only 227 iridate compound, which exhibits a large anomalous Hall effect (AHE) along the [1,1,1] direction below 1.5 K, without possessing any measurable magnetic moment. By focusing on the normal state of 227 iridates, described by a parabolic semimetal with quadratic band touching, we use renormalization group analysis, mean-field theory, and phenomenological Landau theory as three complementary methods to construct a global phase diagram in the presence of generic local interactions among itinerant electrons of Ir ions. While the global phase diagram supports several competing multipolar orders, motivated by the phenomenology of 227 iridates we particularly emphasize the competition between AIAO and SI orders and how it can cause a mixed phase with ``three-in--one-out'' (3I1O) spin configurations. In terms of topological properties of Weyl quasiparticles of the 3I1O state, we provide an explanation for the magnitude and the direction of the observed AHE in ${\mathrm{Pr}}_{2}{\mathrm{Ir}}_{2}{\mathrm{O}}_{7}$. We propose a strain-induced enhancement of the onset temperature for AHE in thin films of ${\mathrm{Pr}}_{2}{\mathrm{Ir}}_{2}{\mathrm{O}}_{7}$ and additional experiments for studying competing orders in the vicinity of the metal-insulator transition. In addition to providing a theory for competing orders and magnetic properties of ${\mathrm{Pr}}_{2}{\mathrm{Ir}}_{2}{\mathrm{O}}_{7}$, the theoretical framework developed in this work should also be useful for a better understanding of competing multipolar orders in other correlated materials.
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Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.002 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.001 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.001 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.000 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it