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Nitrogen Removal from Oil: A Review

2016· review· en· W2567144889 on OpenAlexaff
Glaucia H. C. Prado, Yuan Rao, Arno de Klerk

Bibliographic record

VenueEnergy & Fuels · 2016
Typereview
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsHydrodenitrogenationChemistryHydrodesulfurizationNitrogenCatalysisFuel oilRefining (metallurgy)SolventOrganic chemistryMetalRefineryInorganic chemistryEnvironmental chemistryWaste management

Abstract

fetched live from OpenAlex

Abstract The selective removal of nitrogen-containing compounds from oil and oil fractions is of interest because of the potential deleterious impact of such compounds on products and processes. Problems caused by nitrogen-containing compounds include gum formation, acid catalyst inhibition and deactivation, acid?base pair-related corrosion, and metal complexation. A brief overview of the classes of nitrogen compounds found in oil is provided. The review of processes to remove nitrogen from oil emphasizes studies that investigated denitrogenation of industrial feedstocks, such as refinery fractions, heavy oils, and bitumens. The main topics covered are hydrotreating, liquid?liquid phase partitioning, solvent deasphalting, adsorption, chemical conversion followed by separation, and microbial conversion. Chemical conversion processes include oxidative denitrogenation, N-alkylation, complexation with metal salts, and conversion in high-temperature water. There are many processes for denitrogenation by separation of the nitrogen-rich products from oil without removing the nitrogen group from the nitrogen-containing compounds. As a consequence, most of these processes are viable mainly for removal of nitrogen from low-nitrogen-content oils, typically with <0.1 wt % N. At present, hydrodenitrogenation appears to be the only industrially viable process for nitrogen removal from oils with high nitrogen content.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.006
Threshold uncertainty score0.019

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0040.004
Science and technology studies0.0000.000
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0060.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.264
Teacher spread0.240 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations412
Published2016
Admission routes1
Has abstractyes

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