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Evaluating Diffusivity of Toluene in Heavy Oil Using Nuclear Magnetic Resonance Imaging

2017· article· en· W2570800349 on OpenAlexafffund
Amir Fayazi, Sergey Kryuchkov, Apostolos Kantzas

Bibliographic record

VenueEnergy & Fuels · 2017
Typearticle
Languageen
FieldPhysics and Astronomy
TopicNMR spectroscopy and applications
Canadian institutionsUniversity of Calgary
FundersMaersk OilNatural Sciences and Engineering Research Council of CanadaSuncor Energy IncorporatedAlberta Innovates - Technology FuturesCMG Reservoir Simulation FoundationDevon Energy Corporation
KeywordsTolueneThermal diffusivityDiffusionSolventChemistryRelaxation (psychology)Work (physics)Molecular diffusionMaterials scienceNuclear magnetic resonanceAnalytical Chemistry (journal)ThermodynamicsChromatographyOrganic chemistryPhysics

Abstract

fetched live from OpenAlex

Solvent-based processes have shown technical advantages over thermal techniques for recovery of heavy oil and bitumen. The success of these processes relies on accurate computation of molecular diffusion coefficient which determines how fast a solvent penetrates into oil. Concentration profile measurements of solvent in oil are used for the determination of the molecular diffusion coefficient. Although numerous experimental techniques have been proposed, the accurate estimation of this parameter is still a topic of debate in the literature. In this work, 1-D nuclear magnetic resonance imaging (MRI) is employed to obtain diffusivity data for a toluene–heavy oil system. Diffusion of toluene in heavy oil was monitored for 20 days at a controlled temperature of 35 °C and ambient pressure. Over time, toluene diffusion into oil leads to changes in spatial distribution of T 1 and T 2 that affect the received signal. This serves as the basis of the solvent and heavy oil concentration estimation. Consequently, concentration profiles were established by converting the MRI signals to concentration values. This conversion was achieved by creating samples with known concentrations of heavy oil–toluene and measuring their response in the same environment and parameter settings. A concentration-dependent diffusion coefficient was obtained from concentration profiles. The results show that relaxation based 1D MRI is an accurate and robust tool to obtain diffusivity data in complex fluids such as heavy oil.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.343
Threshold uncertainty score0.532

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.349
Teacher spread0.326 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2017
Admission routes2
Has abstractyes

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