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Determination of the Synergism/Antagonism Parameters during Co-gasification of Potassium-Rich Biomass with Non-biomass Feedstock

2017· article· en· W2574302296 on OpenAlexafffund
Roxin Fernandes, Josephine M. Hill, Jan Kopyscinski

Bibliographic record

VenueEnergy & Fuels · 2017
Typearticle
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsUniversity of CalgaryMcGill University
FundersNatural Sciences and Engineering Research Council of CanadaCarbon Management Canada
KeywordsBiomass (ecology)Raw materialPotassiumChemistryCoalBioenergyPulp and paper industryCarbon fibersBiofuelWaste managementMaterials scienceAgronomyOrganic chemistry

Abstract

fetched live from OpenAlex

This study focuses on quantifying the synergistic/antagonistic behavior occurring during the co-gasification of non-biomass feedstock (ash-free coal and fluid coke) with potassium-rich switchgrass. The results showed that the gasification rate of switchgrass in the mixture decreased as a certain amount of its potassium was transferred to the non-biomass feed, leading to a multifold increase in the non-biomass gasification rate. The aim of this study was to quantify this behavior through kinetic modeling. It was assumed that each constituent in the mixture follows the random pore model with their corresponding kinetic parameters. Furthermore, synergism/antagonism parameters were included, which were either a constant or a function of the switchgrass conversion (linear or square root), representing the effect of interparticle potassium mobility. The acceleration of the gasification rate of the non-biomass feedstock followed a linear function of the switchgrass conversion. The inhibition of the switchgrass conversion did not show a clear trend because it depends upon the non-biomass feedstock and temperature. The presence of potassium in switchgrass, which acts as a catalyst, is clearly observed from the modeling, where the gasification rates for the fluid coke or ash-free coal in the mixture significantly increased for all temperatures studied. Modeling of the gasification reactions with the estimated best fit synergism/antagonism models showed a very good agreement with the observed values. The obtained results of this study can be useful in designing co-gasification systems and estimating the best ratio of biomass/non-biomass feeds.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score0.630

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.213
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations21
Published2017
Admission routes2
Has abstractyes

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