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Record W2594326981 · doi:10.1080/00268976.2017.1297861

Single-laser-induced quantum interference in photofragmentation reaction of D <sup>+</sup> <sub>2</sub>

2017· article· en· W2594326981 on OpenAlexafffund
Chuan‐Cun Shu, Daoyi Dong, Kai‐Jun Yuan

Bibliographic record

VenueMolecular Physics · 2017
Typearticle
Languageen
FieldPhysics and Astronomy
TopicLaser-Matter Interactions and Applications
Canadian institutionsUniversité de Sherbrooke
FundersAustralian Research CouncilCompute CanadaUniversity of New South Wales Canberra
KeywordsConical intersectionAtomic physicsDiatomic moleculeKinetic energyIonic bondingQuantumLaserChemistryPhysicsInterference (communication)IonPotential energyOpticsMoleculeQuantum mechanics

Abstract

fetched live from OpenAlex

We theoretically study quantum interference phenomena in the photofragmentation reaction of breaking up the diatomic molecular ion D+ 2 into an atom D and an ionic D+ by a single ultrashort laser pulse. The numerical results show that the occurrence of quantum interference in kinetic energy release spectra is sensitive to the angle between the molecular axis and the laser field polarisation direction. Such sensitivity is shown to be dependent on the initial vibrational quantum state of the system and the pulse intensity. The underlying mechanism for the single-pulse-induced quantum interference is analysed by using a light-induced potential and light-induced conical intersection concept.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.035
Threshold uncertainty score0.707

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.272
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2017
Admission routes2
Has abstractyes

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