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Record W2604154480 · doi:10.1002/celc.201700214

High Capacitance and Cycle‐Life Performance of a Binder‐Free Supercapacitor Nanocomposite Electrode by Direct Growth of Manganese Oxide Nanostructures on Carbon Nanotubes

2017· article· en· W2604154480 on OpenAlexafffund
Fatemeh Ataherian, Youling Wang, Amel Tabet‐Aoul, Mohamed Mohamedi

Bibliographic record

VenueChemElectroChem · 2017
Typearticle
Languageen
FieldMaterials Science
TopicSupercapacitor Materials and Fabrication
Canadian institutionsInstitut National de la Recherche Scientifique
FundersNatural Sciences and Engineering Research Council of CanadaChina Scholarship CouncilCentre québécois sur les matériaux fonctionnels
KeywordsHorizontal scan rateMaterials scienceSupercapacitorNanocompositeCapacitanceCyclic voltammetryDielectric spectroscopyX-ray photoelectron spectroscopyElectrochemistryCarbon nanotubeScanning electron microscopeElectrolyteChemical engineeringElectrodeNanotechnologyAnalytical Chemistry (journal)Composite materialChemistry

Abstract

fetched live from OpenAlex

Abstract MnOx thin films with various oxidation states (MnO, Mn2O3, MnO2 and mixed MnO/Mn3O4) were directly grown onto carbon nanotubes by pulsed laser deposition under vacuum and at different oxygen partial pressures. The microstructural features of the as‐deposited thin films are characterized by scanning electron microscopy and X‐ray photoelectron spectroscopy. The electrochemical behavior of the CNT/MnOx nanocomposites in 1 M Na2SO4 electrolyte is discussed with regards to specific capacitance, and cycle‐life, by means of cyclic voltammetry and electrochemical impedance measurements. First, at slow potential scan rate of 1 mV s−1, MnOx prepared under vacuum and 10 mTorr of O2 delivered specific capacitance as high as 738 and 653 F g−1, respectively. Second, the rate capability of these two nanocomposites over a wide range of scan rates showed that at 500 mV s−1, the former retained 93 % whereas the later displayed an increase of 1.2 % with regards to their respective initial specific capacitance values at 1 mV s−1. They also maintained 90 % and 95 % of their specific capacitance after 10 000 continuous cycles with a 100 mV s−1 scan rate. The binder‐free nature of the CNT/MnOx nanocomposites and remarkable electrochemical properties suggest that these materials could find application as excellent electrodes for supercapacitors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.199
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2017
Admission routes2
Has abstractyes

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