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Record W2607279442 · doi:10.1002/cjce.22861

Wood sawdust and sewage sludge pyrolysis chars for CO<sub>2</sub> adsorption using a magnetic suspension balance

2017· article· en· W2607279442 on OpenAlexvenueno aff
Paula Fabiane Pinheiro do Nascimento, João Fernandes de Sousa, Jackson Araújo de Oliveira, Rosangela D. Possa, Luciene Santos de Carvalho, Fabíola C. Carvalho, Juan A.C. Ruiz, Marcelo Mendes Pedroza, M. B. D. Bezerra

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2017
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsnot available
Fundersnot available
KeywordsSawdustFreundlich equationPotassium hydroxideAdsorptionSewage sludgePyrolysisSpecific surface areaCharChemistryDichloromethanePulp and paper industryLangmuirVolume (thermodynamics)DesorptionChemical engineeringEnvironmental chemistryWaste managementSewage treatmentSolventOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

Abstract In view of global warming caused by the uncontrolled emissions of CO 2 to the environment, there is a great need to develop methods able to eliminate this pollutant. Apart from establishing new techniques, the exploration of new materials with high separation performance and low cost are of importance. This work aims to treat carbon‐metals‐rich chars originated from the fast pyrolysis of sewage sludge and wood sawdust to be used as CO 2 adsorbents. The samples were washed with ethanol and dichloromethane before their physical and chemical activation to remove impregnated bio‐oil. For the chemical activation, potassium hydroxide and hydrochloric acid were used as agents. The samples were analyzed via BET, TGA, XRD, and XRF. The results were used to investigate the role played by ethanol or dichloromethane and the effect of the activation on the properties of the materials such as specific surface area, total specific pore volume, and average pore size. CO 2 isotherms were obtained experimentally at 25 °C using a magnetic suspension balance and the data was used to estimate Langmuir and Freundlich isotherm parameters. After chemical treatment, the sewage sludge char specific surface area increased 11 times and had an adsorptive capacity of 1.32 × 10 −3 mol/g. The wood sawdust char specific surface area increased 90 times and had an adsorptive capacity of 3.73 × 10 −3 mol/g. Desorption was carried out from 5 × 10 5 to 1 × 10 5 Pa at 37 °C and the efficiencies were 89.0 and 84.4 % for the sewage sludge and wood sawdust, respectively.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.095
Threshold uncertainty score0.662

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.197
Teacher spread0.186 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations18
Published2017
Admission routes1
Has abstractyes

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