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Record W2623263030 · doi:10.1038/s41598-017-03839-x

A Facile Green Synthetic Route for the Preparation of Highly Active γ-Al2O3 from Aluminum Foil Waste

2017· article· en· W2623263030 on OpenAlexfundno aff
Ahmed I. Osman, Jehad K. Abu‐Dahrieh, Mathew McLaren, Fathima Laffir, Peter Nockemann, David W. Rooney

Bibliographic record

VenueScientific Reports · 2017
Typearticle
Languageen
FieldMaterials Science
TopicMagnesium Oxide Properties and Applications
Canadian institutionsnot available
FundersSouth Valley UniversityQueen's UniversityQueen's University Belfast
KeywordsCatalysisMonoclinic crystal systemFOIL methodMesoporous materialMaterials scienceDimethyl etherMethanolCrystal structureNuclear chemistryChemical engineeringInorganic chemistryChemistryOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Abstract A novel green preparation route to prepare nano-mesoporous γ-Al2O3 from AlCl3.6H2O derived from aluminum foil waste and designated as ACFL550 is demonstrated, which showed higher surface area, larger pore volume, stronger acidity and higher surface area compared to γ-Al2O3 that is produced from the commercial AlCl3 precursor, AC550. The produced crystalline AlCl3.6H2O and Al(NO3)3.9H2O in the first stage of the preparation method were characterized by single-crystal XRD, giving two crystal structures, a trigonal (R-3c) and monoclinic (P21/c) structure, respectively. EDX analysis showed that ACFL550 had half the chlorine content (Cl%) relative to AC550, which makes ACFL550 a promising catalyst in acid-catalysed reactions. Pure and modified ACFL550 and AC550 were applied in acid-catalysed reactions, the dehydration of methanol to dimethyl ether and the total methane oxidation reactions, respectively. It was found that ACFL550 showed higher catalytic activity than AC550. This work opens doors for the preparation of highly active and well-structured nano-mesoporous alumina catalysts/supports from aluminum foil waste and demonstrates its application in acid-catalysed reactions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.276
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations59
Published2017
Admission routes1
Has abstractyes

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Same venueScientific ReportsSame topicMagnesium Oxide Properties and ApplicationsFrench-language works237,207