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Record W2625359408 · doi:10.1021/acs.iecr.7b01123

Pyrolysis Kinetics of Pre-Torrefied Woody Biomass Based on Torrefaction Severity—Experiments and Model Verification

2017· article· en· W2625359408 on OpenAlexafffund
A. Sarvaramini, Faı̈çal Larachi

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2017
Typearticle
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsUniversité Laval
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsTorrefactionPyrolysisBiomass (ecology)HemicelluloseCellulosePulp and paper industryLigninRaw materialThermogravimetryLignocellulosic biomassMaterials scienceSawdustChemical engineeringChemistryOrganic chemistryAgronomy

Abstract

fetched live from OpenAlex

A kinetic model was developed for the pyrolysis of pre-torrefied lignocellulosic biomass requiring solely knowledge of the pyrolysis kinetics of raw biomass. To predict yield and differential thermogravimetry (DTG) profiles for the pyrolysis of pre-torrefied biomass specimens, the classical three-parallel first-order pyrolysis kinetic model was modified to incorporate severity factors accounting for the impact of torrefaction time and temperature on the devolatilization of hemicellulose, cellulose, and lignin biomass components. The model also included features to account for the effect of pyrolysis heating rate on pyrolysis activation energies of the biomass components both for raw and pre-torrefied substrates. Specifically, severity factor correlations between pre-torrefaction conditions and biomass component relative weights prior to pyrolysis were developed so that the kinetic model, validated at the outset for the pyrolysis of raw biomass specimens, could also be applicable for the pre-torrefied samples. Thermal decompositions of raw and pre-torrefied birch, aspen, and sawdust specimens were tested through thermogravimetric analyses under various pyrolysis heating rates and isothermal torrefaction exposure times and temperatures. Model confrontation against pyrolysis yields and DTG rates measured at varying severities for both raw and pre-torrefied woody biomass confirmed that predicted pyrolysis yields and rates were in a good agreement with experiments.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.193
Threshold uncertainty score0.906

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.072
GPT teacher head0.321
Teacher spread0.249 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2017
Admission routes2
Has abstractyes

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