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Record W2729157071 · doi:10.1021/acs.iecr.7b01445

Site Energy Distribution and X-ray Analyses of Nickel Loaded on Heterogeneous Adsorbents

2017· article· en· W2729157071 on OpenAlexafffund
Bei Yan, Catherine Hui Niu, Renfei Feng

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2017
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsCanadian Light Source (Canada)University of Saskatchewan
FundersAgriculture and Agri-Food CanadaNatural Sciences and Engineering Research Council of CanadaChina Scholarship CouncilCanada Foundation for InnovationMinistry of Agriculture - Saskatchewan
KeywordsAdsorptionNickelAbsorption (acoustics)LangmuirMoleculeFreundlich equationChemistryMaterials scienceExtended X-ray absorption fine structureAnalytical Chemistry (journal)Inorganic chemistryPhysical chemistryAbsorption spectroscopyChromatographyOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

The approximate site energy distributions were estimated to describe the adsorption of nickel ions on the heterogeneous surfaces of barley straw adsorbents based on the Langmuir–Freundlich model. The average site energy and standard deviation of the site energy distributions of the adsorbents were determined to analyze the interaction between the adsorbents and adsorbate, and the adsorption site heterogeneity. With higher site energy, the pretreated barley straw (PBS) has higher nickel adsorption capacity (59.5 mg/g) than most of the reported adsorbents. The bonding of nickel on PBS was investigated by X-ray absorption spectroscopies. X-ray absorption near edge structure results indicated that the nickel adsorbed on PBS remained as Ni(II). Extended X-ray absorption fine structure data indicated that the adsorbed Ni was bonded to 6 oxygen atoms of carboxyl groups and/or water molecules. The results and methodology in this work are transferable to investigate other adsorption systems for separation applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.107
GPT teacher head0.349
Teacher spread0.242 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2017
Admission routes2
Has abstractyes

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Same venueIndustrial & Engineering Chemistry ResearchSame topicAdsorption and biosorption for pollutant removalFrench-language works237,207