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Record W2732944238 · doi:10.1038/s41598-017-03714-9

Gasoline cars produce more carbonaceous particulate matter than modern filter-equipped diesel cars

2017· article· en· W2732944238 on OpenAlexaff
Stephen M. Platt, Imad El Haddad, Simone M. Pieber, Alessandro Zardini, Ricardo Suárez‐Bertoa, Michaël Clairotte, Kaspar R. Daellenbach, Ru‐Jin Huang, Jay G. Slowik, Stig Hellebust, Brice Temime‐Roussel, Nicolas Marchand, J. A. de Gouw, J. L. Jiménez, Patrick L. Hayes, Allen L. Robinson, Urs Baltensperger, Covadonga Astorga, Andrê S. H. Prévôt

Bibliographic record

VenueScientific Reports · 2017
Typearticle
Languageen
FieldEnvironmental Science
TopicAir Quality and Health Impacts
Canadian institutionsUniversité de Montréal
FundersNational Institute of Environmental Health SciencesEuropean CommissionAix-Marseille UniversitéSchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen ForschungU.S. Environmental Protection AgencyBundesamt für UmweltAgence de l'Environnement et de la Maîtrise de l'EnergieNational Science Foundation
KeywordsGasolineDiesel fuelParticulatesEnvironmental scienceAerosolDiesel exhaustAir pollutionPollutantDiesel particulate filterPollutionWaste managementEnvironmental engineeringEnvironmental chemistryChemistryEngineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Carbonaceous particulate matter (PM), comprising black carbon (BC), primary organic aerosol (POA) and secondary organic aerosol (SOA, from atmospheric aging of precursors), is a highly toxic vehicle exhaust component. Therefore, understanding vehicle pollution requires knowledge of both primary emissions, and how these emissions age in the atmosphere. We provide a systematic examination of carbonaceous PM emissions and parameterisation of SOA formation from modern diesel and gasoline cars at different temperatures (22, −7 °C) during controlled laboratory experiments. Carbonaceous PM emission and SOA formation is markedly higher from gasoline than diesel particle filter (DPF) and catalyst-equipped diesel cars, more so at −7 °C, contrasting with nitrogen oxides (NO X ). Higher SOA formation from gasoline cars and primary emission reductions for diesels implies gasoline cars will increasingly dominate vehicular total carbonaceous PM, though older non-DPF-equipped diesels will continue to dominate the primary fraction for some time. Supported by state-of-the-art source apportionment of ambient fossil fuel derived PM, our results show that whether gasoline or diesel cars are more polluting depends on the pollutant in question, i.e. that diesel cars are not necessarily worse polluters than gasoline cars.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesScience and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.092
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0020.001
Scholarly communication0.0010.001
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.039
GPT teacher head0.309
Teacher spread0.270 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations203
Published2017
Admission routes1
Has abstractyes

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