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Record W2734519455 · doi:10.1002/pola.28713

Functionalization of polyesters with multiple B vitamins

2017· article· en· W2734519455 on OpenAlexaff
Andrew G. Soxman, Jenna M. DeLuca, Kylie M. Kinlough, David F. Iwig, Robert T. Mathers

Bibliographic record

VenueJournal of Polymer Science Part A Polymer Chemistry · 2017
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsKensington Health
FundersNational Science Foundation
KeywordsChemistryCovalent bondMonomerPolymerizationPolymer chemistryThermal stabilitySolubilitySolventOrganic chemistryDiketeneSurface modificationPolymer

Abstract

fetched live from OpenAlex

ABSTRACT A method to covalently attach combinations of six different B vitamins provided an avenue to new functional thermosets without multi‐step coupling reactions. The melt polymerization strategy required no organic solvent and facilitated covalent attachment of OH (B1, B2, B5, B6) or COOH (B7, B9) groups on B vitamins via Fischer esterification. Characterization of model reactions with LC/MS, FTIR, and GPC confirmed covalent attachment. Based on control experiments, B vitamins demonstrated unexpected thermal stability and appreciable solubility in the melt polymerization. This approach was demonstrated with citric acid and diglycerol, but has wide‐ranging potential for other polar monomers with negative octanol–water partition coefficients (LogP). © 2017 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2017, 55, 3308–3316

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.236
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2017
Admission routes1
Has abstractyes

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