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Record W2747417738 · doi:10.1080/1478422x.2017.1297575

The kinetics of film growth and their influence on the susceptibility to pitting of copper in aqueous sulphide solutions

2017· article· en· W2747417738 on OpenAlexaff
Taylor Martino, Jian Chen, Z. Qin, David W. Shoesmith

Bibliographic record

VenueCorrosion Engineering Science and Technology The International Journal of Corrosion Processes and Corrosion Control · 2017
Typearticle
Languageen
FieldMaterials Science
TopicCorrosion Behavior and Inhibition
Canadian institutionsWestern University
FundersSvensk Kärnbränslehantering
KeywordsCopperCorrosionAqueous solutionChloridePitting corrosionErosion corrosion of copper water tubesElectrolyteElectrochemistryMetallurgyMaterials sciencePassivityKineticsPorosityInorganic chemistryChemistryElectrodeComposite material

Abstract

fetched live from OpenAlex

The formation of copper sulphide films on copper in aqueous sulphide solutions has been investigated under both natural corrosion and electrochemical conditions. Film growth occurs at the Cu2S/electrolyte interface and involves Cu+ transport through a generally porous film. Both corrosion and anodic film growth are suppressed by high chloride concentrations. Passivity, a pre-requisite for pitting, is achievable only at high sulphide concentrations and transport fluxes, conditions not expected under most geologic repository conditions since both sulphide groundwater concentrations and diffusive transport rates are expected to be low.This paper is part of a supplement on the 6th International Workshop on Long-Term Prediction of Corrosion Damage in Nuclear Waste Systems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.006
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score0.721

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.006
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.240
Teacher spread0.231 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations38
Published2017
Admission routes1
Has abstractyes

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