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Record W2751062572 · doi:10.1021/acs.iecr.7b01708

Conversion of Wood-Based Hemicellulose Prehydrolysate into Succinic Acid Using a Heterogeneous Acid Catalyst in a Biphasic System

2017· article· en· W2751062572 on OpenAlexafffund
Sai Swaroop Dalli, Tewodros Jemberu Tilaye, Sudip Kumar Rakshit

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2017
Typearticle
Languageen
FieldEngineering
TopicCatalysis for Biomass Conversion
Canadian institutionsLakehead University
FundersCanada Research ChairsCanada Foundation for Innovation
KeywordsFurfuralHemicelluloseSuccinic acidChemistryAcetic acidYield (engineering)Organic chemistryCatalysisTolueneCelluloseMaterials science

Abstract

fetched live from OpenAlex

A novel approach for the conversion of biomass-based hemicellulose prehydrolysate to high-value succinic acid has been investigated using a heterogeneous acid catalyst, Amberlyst 15 and hydrogen peroxide, in a biphasic system. A vital intermediate in this process, furfural, was oxidized in the biphasic system to produce succinic acid. Production of furfural in good yields is a limiting step in such processes for a number of reasons. Among the organic solvents evaluated, toluene was found to be an ideal solvent for furfural extraction and to facilitate the conversion of furfural to succinic acid. Simultaneous extraction of furfural into the organic solvent as it was produced increased the overall yield. It was observed that the developed method resulted in a succinic acid yield of 52.34% from the furfural obtained from hemicellulose prehydrolysate. It was found that 50 mg of Amberlyst 15 per millimole of furfural resulted in 100% furfural conversion in less time.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.057
GPT teacher head0.296
Teacher spread0.239 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2017
Admission routes2
Has abstractyes

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