MétaCan
Menu
Back to cohort
Record W2753025542 · doi:10.1021/acschembio.7b00481

Selective Targeting of Bromodomains of the Bromodomain-PHD Fingers Family Impairs Osteoclast Differentiation

2017· article· en· W2753025542 on OpenAlexafffund
Julia Meier, C. Tallant, Oleg Fedorov, Hanna Witwicka, Sung‐Yong Hwang, Ruud GPM van Stiphout, Jean‐Philippe Lambert, Catherine Rogers, Clarence Yapp, Brian S. Gerstenberger, Vita Fedele, P. Savitsky, David Heidenreich, Danette L. Daniels, Dafydd R. Owen, Paul V. Fish, Niall Igoe, Elliott D. Bayle, Bernard Haendler, Udo Oppermann, Francesca M. Buffa, Paul E. Brennan, Susanne Müller, Anne‐Claude Gingras, Paul R. Odgren, Mark J. Birnbaum, Stefan Knapp

Bibliographic record

VenueACS Chemical Biology · 2017
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicProtein Degradation and Inhibitors
Canadian institutionsUniversity of TorontoMount Sinai HospitalLunenfeld-Tanenbaum Research InstituteStructural Genomics Consortium
FundersNational Institute of Dental and Craniofacial ResearchMedical Research CouncilCanadian Institutes of Health ResearchNational Institute of Arthritis and Musculoskeletal and Skin DiseasesRosetrees TrustVersus ArthritisArthritis Research UKTD BankCancer Research UKWellcome TrustBayer
KeywordsBromodomainOsteoclastBiologyCell biologyChemistryComputational biologyGeneticsAcetylationGeneIn vitro

Abstract

fetched live from OpenAlex

Histone acetyltransferases of the MYST family are recruited to chromatin by BRPF scaffolding proteins. We explored functional consequences and the therapeutic potential of inhibitors targeting acetyl-lysine dependent protein interaction domains (bromodomains) present in BRPF1-3 in bone maintenance. We report three potent and selective inhibitors: one (PFI-4) with high selectivity for the BRPF1B isoform and two pan-BRPF bromodomain inhibitors (OF-1, NI-57). The developed inhibitors displaced BRPF bromodomains from chromatin and did not inhibit cell growth and proliferation. Intriguingly, the inhibitors impaired RANKL-induced differentiation of primary murine bone marrow cells and human primary monocytes into bone resorbing osteoclasts by specifically repressing transcriptional programs required for osteoclastogenesis. The data suggest a key role of BRPF in regulating gene expression during osteoclastogenesis, and the excellent druggability of these bromodomains may lead to new treatment strategies for patients suffering from bone loss or osteolytic malignant bone lesions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.390

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.244
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations56
Published2017
Admission routes2
Has abstractyes

Explore more

Same venueACS Chemical BiologySame topicProtein Degradation and InhibitorsFrench-language works237,207