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Record W2756323147 · doi:10.1021/acs.cgd.7b01015

Unprecedented Octanuclear Dy<sup>III</sup> Cluster Exhibiting Single-Molecule Magnet Behavior

2017· article· en· W2756323147 on OpenAlexafffund
Thomas Lacelle, Gabriel Brunet, Rebecca J. Holmberg, Bulat Gabidullin, Muralee Murugesu

Bibliographic record

VenueCrystal Growth & Design · 2017
Typearticle
Languageen
FieldMaterials Science
TopicMagnetism in coordination complexes
Canadian institutionsUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of CanadaCanada Foundation for InnovationUniversity of Ottawa
KeywordsCubaneCrystallographyChemistryMagnetizationCluster (spacecraft)MoietyMoleculeRelaxation (psychology)MagnetSingle-molecule magnetQuantum tunnellingNuclear magnetic resonanceCondensed matter physicsStereochemistryMagnetic fieldCrystal structurePhysics

Abstract

fetched live from OpenAlex

An unprecedented Dy 8 cluster, [Dy 8 (μ 4 -O)(μ 3 -OH) 8 (vht) 4 (NO 3 ) 2 (H 2 O) 8 ](NO 3 ) 4, composed of two fused and distorted [Dy 4 (μ 3 -OH) 4 ] 8+ cubane units is reported. The bridging of the two cubanes occurs through a planar μ 4 -O (oxide) moiety, and leads to the largest reported distortion of the Dy-O-Dy angles within a [Dy 4 (OH) 4 ] cubane core. In turn, this leads to clear zero-field slow relaxation of the magnetization, characteristic of single-molecule magnets (SMMs). Further magnetic analyses suggest that the relaxation may be largely dictated by quantum tunneling of the magnetization and Raman processes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Scholarly communication, Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.055
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0020.001
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.266
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2017
Admission routes2
Has abstractyes

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