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Record W2767315881 · doi:10.1149/2.1831713jes

Effect of Oxide Film Properties on the Kinetics of O<sub>2</sub>Reduction on Alloy C-22

2017· article· en· W2767315881 on OpenAlexafffund
Xiangrong Zhang, Zack Qin, Dmitrij Zagidulin, James J. Noël, David W. Shoesmith

Bibliographic record

VenueJournal of The Electrochemical Society · 2017
Typearticle
Languageen
FieldMaterials Science
TopicCorrosion Behavior and Inhibition
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsAlloyKineticsReduction (mathematics)OxideMaterials scienceChemical engineeringMetallurgyAnalytical Chemistry (journal)ChemistryPhysicsMathematicsChromatographyEngineeringGeometry

Abstract

fetched live from OpenAlex

The kinetics of oxygen reduction have been studied electrochemically on the Ni-Cr-Mo(W) Alloy C-22 in 5 M NaCl at 70°C using potentiostatic and voltammetric techniques and electrochemical impedance spectroscopy. Oxygen reduction was observed to occur at low potentials on defective oxide films containing a high concentration of anion vacancies and appeared to proceed by a combination of 2-electron and 4-electron transfer processes. At more positive potentials a passive film comprising a Cr III -dominated barrier layer at the alloy/oxide interface and a Mo/W enriched outer layer at the oxide/solution interface was formed, and oxygen reduction was completely suppressed. Oxygen reduction could be revived after transpassive degradation of the oxide film at more positive potentials, and appeared to be catalyzed on the Mo VI /W VI surface film.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.241
Teacher spread0.228 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2017
Admission routes2
Has abstractyes

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Same venueJournal of The Electrochemical SocietySame topicCorrosion Behavior and InhibitionFrench-language works237,207