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Record W2768800606

Re-Os Systematics of Crude Oil and Re-Os Petroleum System Geochronology

2017· dissertation· en· W2768800606 on OpenAlex
Junjie Liu

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

aboutThe title or abstract carries a Canadian signal from the geographic lexicon.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueDurham e-Theses (Durham University) · 2017
Typedissertation
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsnot available
Fundersnot available
KeywordsAsphaltenePetroleumGeochronologyGeologyThermal ionization mass spectrometrySource rockGeochemistryIsotopeMineralogyIsotope dilutionMass spectrometryStructural basinChemistryPaleontologyChromatographyIon sourceNuclear physics
DOInot available

Abstract

fetched live from OpenAlex

Re and Os are present in many crude oils in measurable abundances. The Re-Os geochronometer has successfully constrained the timing of oil generation, thermochemical sulphate reduction and thermal alteration of crude oil for petroleum systems worldwide. The Os isotope composition has also been used as an oil-source correlation tool.
\nThis thesis firstly presents two petroleum matrix-matched Re-Os measurement reference materials: the RM8505 crude oil and ~ 90 g homogeneous asphaltene powder isolated from the RM8505 crude oil. The Re-Os data are from the repeated measurements of these samples via the Carius Tube - Isotope Dilution - Negative Thermal Ionization Mass Spectrometry methodology. The normal distribution and low relative standard deviation of the abundance and isotopic data ensure them to be appropriate petroleum matrix-matched reference materials for Re-Os measurements.
\nA Re-Os age of 66 ± 31 Ma was defined by the Duvernay-sourced oil asphaltene fractions from Western Canada sedimentary basin. This age is in excellent agreement with the main-stage hydrocarbon generation of Duvernay Formation based on basin modelling. Further, this study supports Os isotope composition as a valid oil-source tracer and the hypothesis that the oil 187Os/188Os composition is inherited from the source unit during oil generation. This study shows limited or no influence of the Re-Os systematics of crude oil through the interaction of basinal fluids.
\nThe progressively precipitated asphaltene fractions of six oil samples exhibit a decrease in Re and Os abundance, and diverse 187Re/188Os and 187Os/188Os patterns. This study proposes that Re and Os in crude oil are to be bound in multiple free compounds and such molecules occluded/absorbed in the asphaltene aggregate structure. No combination of the fractions of a crude oil can consistently yield geologically meaningful Re-Os age for all of the six oil samples, either the progressively precipitated asphaltene fractions or the asphaltenes and maltenes separated by n-alkanes. As such, obtaining geologically meaningful Re-Os dates from a single oil may not be viable for many oils.
\n

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.550
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.206
Teacher spread0.194 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it