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Record W2769504886 · doi:10.1021/acs.jpcc.7b08978

Short-Range Structure of TeO<sub>2</sub> Glass

2017· article· en· W2769504886 on OpenAlexafffund
Mounesha N. Garaga, Ulrike Werner‐Zwanziger, Josef W. Zwanziger, Anthony V. DeCeanne, Brittney M. Hauke, K. Bozer, Steve Feller

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2017
Typearticle
Languageen
FieldMaterials Science
TopicGlass properties and applications
Canadian institutionsDalhousie University
FundersDivision of Materials ResearchNatural Sciences and Engineering Research Council of CanadaCompute CanadaNational Science Foundation
KeywordsRaman spectroscopyCrystal (programming language)Crystal structureMaterials scienceCrystallographyDiffractionSpectroscopyRange (aeronautics)Solid-stateChemistryAnalytical Chemistry (journal)OpticsPhysical chemistryPhysics

Abstract

fetched live from OpenAlex

The short-range structure of TeO 2 glass was studied by a combined solid-state NMR, Raman, and first-principles calculation approach. Glass samples enriched in oxygen-17 were prepared, and both 125 Te and 17 O spectra were recorded. In addition, spectra of α-TeO 2 and γ-TeO 2 crystal phases were recorded to aid in spectral assignment. The identity of the crystal phases was confirmed by X-ray diffraction and Raman spectroscopy. First-principles computations on the TeO 2 crystal phases as well as on several potassium tellurites were carried out for comparison. It was found that the structure of TeO 2 glass is best described as a highly disordered form of the γ-TeO 2 crystal.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.249
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations45
Published2017
Admission routes2
Has abstractyes

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Same venueThe Journal of Physical Chemistry CSame topicGlass properties and applicationsFrench-language works237,207