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Record W2772187827

Inhibition of Holocellulose Active Enzymes due to Steric Hindrances and Non-specific Binding on Lignocellulose Surfaces

2016· dissertation· en· W2772187827 on OpenAlexfundno aff

Bibliographic record

VenueTSpace (University of Toronto) · 2016
Typedissertation
Languageen
FieldEngineering
TopicLignin and Wood Chemistry
Canadian institutionsnot available
FundersUniversity of Toronto
KeywordsSteric effectsEnzymeChemistryBiochemistryStereochemistry
DOInot available

Abstract

fetched live from OpenAlex

The adsorption of xylanases from Thermobifida fusca (TfuXyn10B and TfuXyn11A) onto lignin samples derived from kraft and organosolv pulping processes was monitored using a quartz crystal microbalance with dissipation (QCM-D). While TfuXyn11A comprises a C-terminal family 2b carbohydrate-binding module (CBM) and bound to lignin surfaces, TfuXyn10B lacking a CBM did not bind any lignin source. Pretreatment with bovine serum albumin effectively prevented TfuXyn11A adsorption. Enzyme adsorption was limited to a surface interaction and did not lead to swelling of the lignin coating. A novel approach was developed to distinguish between the mass of protein and protein-bound water binding to the lignin surfaces. Kinetic analysis of enzyme association and dissociation revealed that kinetics driving desorption of TfuXyn11A from each lignin source were similar. By contrast, the adsorption kinetics was highest for TfuXyn11A binding to kraft lignin. A lignocellulose composite surface composed of lignin, cellulose and xylan was developed to study impedance of cellulase action

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.201
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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Same venueTSpace (University of Toronto)Same topicLignin and Wood ChemistryFrench-language works237,207