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Determination of the Acetyl Group in Biomass and Its Products by Headspace Gas Chromatography

2017· article· en· W2774202206 on OpenAlexaff
Hui‐Chao Hu, Shaokai Zhang, Tong Zeng, Na Wu, Yonghao Ni, Liulian Huang, Lihui Chen, Xin‐Sheng Chai

Bibliographic record

VenueEnergy & Fuels · 2017
Typearticle
Languageen
FieldEngineering
TopicBiofuel production and bioconversion
Canadian institutionsUniversity of New Brunswick
FundersFujian Provincial Department of Science and TechnologyMinistry of Science and Technology of the People's Republic of ChinaDepartment of Education, Fujian ProvinceNational Natural Science Foundation of China
KeywordsChromatographyChemistryGas chromatographyOxalic acidBiomass (ecology)BiorefineryAcetic acidDetection limitSample preparationAnalytical Chemistry (journal)Organic chemistry

Abstract

fetched live from OpenAlex

This paper reports on a robust method to quantify the acetyl group in biomass and its derived liquid or solid samples using headspace gas chromatography (HS–GC). The method was based on the sample pretreatment in an oxalic acid medium (0.6 mol/L) at 150 °C and 10 min for the liquid samples or 70 min for the solid samples to convert the acetyl group to acetic acid, which can be quantified by a full evaporation HS–GC technique. It was found that ∼100 μm was the suitable solid particle size to be used in the sample analysis at the suggested pretreatment condition. The results showed that the present method has good measurement precision (relative standard deviation was less than 2.09% for the liquid sample and 2.83% for the solid sample) and accuracy (with the recoveries of 96.2–104% in the acetyl group quantification). The limit of quantification of the method was 163 mg/L for the biomass liquid samples and 0.11% for the biomass solid samples. The present method can be a valuable tool to provide the high-throughput testing for the acetyl group in biomass and its derived samples in biorefinery-related development.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.203
Teacher spread0.194 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2017
Admission routes1
Has abstractyes

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