Metal‐Organic‐Framework‐Derived Co Nanoparticles Deposited on N‐Doped Bimodal Mesoporous Carbon Nanorods as Efficient Bifunctional Catalysts for Rechargeable Zinc−Air Batteries
Why this work is in the frame
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Bibliographic record
Abstract
Abstract Electrically rechargeable zinc−air batteries (ZnABs) have received increasing attention as promising energy storage devices, owing to their high theoretical energy density and environmental friendliness. However, it remains a great challenge to develop highly efficient bifunctional catalysts for the oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). Herein, we design and prepare a highly active bifunctional catalyst for ZnABs by using a cobalt metal‐organic framework (Co‐MOF) as the precursor. The catalyst has a desirable nanostructure composed of cobalt nanoparticles deposited on N‐doped bimodal mesoporous carbon nanorods (Co@N‐CNR). This hybrid structure exhibits a higher catalytic activity (a maximum power density of 63 mW cm −2 ) and cycling stability compared to commercial Pt/C+Ir/C integrated in ZnABs . The high catalytic performance could be attributed to the unique nanostructure composed of Co@N‐CNR, which incorporates the advantageous features of cobalt nanoparticles, mesoporous materials, and N‐CNR towards OER and ORR. The reported advancement provides a new and efficient strategy for the development of rechargeable ZnABs.
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Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.001 |
| Science and technology studies | 0.000 | 0.000 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.001 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.000 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it