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Record W2783261276 · doi:10.1002/9781119235941.ch9

Catenated Germanium and Tin Oligomers and Polymers

2017· other· en· W2783261276 on OpenAlexafffund
Daniel A. Foucher

Bibliographic record

Venuenot available
Typeother
Languageen
FieldChemistry
TopicSynthesis and characterization of novel inorganic/organometallic compounds
Canadian institutionsToronto Metropolitan University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsGermaniumTinChromophorePolymerCombinatorial chemistryElectrochemistryCoupling (piping)Materials scienceChemistryNanotechnologyPolymer chemistryOrganic chemistryPhysical chemistryElectrodeMetallurgySilicon

Abstract

fetched live from OpenAlex

This chapter details the innovative chemistry and interesting structural and electronic properties of later Group 14 (Ge, Sn) oligomers and polymers that has been revealed over the last 25-30 years. The common reductive coupling methods used for the synthesis of polygermanes include Wurtz type or electrochemical coupling of dialkyl and diaryl germanium dichlorides. Reductive coupling has also been demonstrated for low-valent dihaloger manes. Alternatively, the coupling of methylated germanes via demethylative processes in the presence of a transition metal catalyst is another successful route to materials of this type. High molecular weight examples of both polygermanes and polystannanes have been prepared by a number of synthetic methods; however, their sensitivity to moisture and light sources has hindered extensive testing and applications. New methodologies and strategies designed for both polymeric systems that effectively counter light-sensitivity have been approached with the use of dyes and attached chromophores.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.026

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0080.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.218
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2017
Admission routes2
Has abstractyes

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