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Record W2789038694 · doi:10.1103/physrevb.97.045424

Quasi-two-dimensional thermoelectricity in SnSe

2018· article· en· W2789038694 on OpenAlexafffund
V. Tayari, Boris V. Senkovskiy, Dmitry V. Rybkovskiy, Niels Ehlen, А.А. Федоров, C.-Y. Chen, J. Ávila, M. C. Asensio, A. Perucchi, Paola Di Pietro, Lada V. Yashina, Ibrahim Fakih, N. Hemsworth, M. Petrescu, G. Gervais, A. Grüneis, Thomas Szkopek

Bibliographic record

VenuePhysical review. B./Physical review. B · 2018
Typearticle
Languageen
FieldMaterials Science
TopicAdvanced Thermoelectric Materials and Devices
Canadian institutionsMcGill University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanadian Institute for Advanced ResearchDeutsche ForschungsgemeinschaftU.S. Department of EnergyEuropean Research CouncilNational Science Foundation
KeywordsSeebeck coefficientThermoelectric effectCondensed matter physicsSemiconductorMaterials scienceThermoelectric materialsDopingSpectroscopyValence (chemistry)Electron mobilityElectrical resistivity and conductivityOptoelectronicsChemistryPhysicsThermodynamics

Abstract

fetched live from OpenAlex

Stannous selenide is a layered semiconductor that is a polar analog of black phosphorus and of great interest as a thermoelectric material. Unusually, hole doped SnSe supports a large Seebeck coefficient at high conductivity, which has not been explained to date. Angle-resolved photoemission spectroscopy, optical reflection spectroscopy, and magnetotransport measurements reveal a multiple-valley valence-band structure and a quasi-two-dimensional dispersion, realizing a Hicks-Dresselhaus thermoelectric contributing to the high Seebeck coefficient at high carrier density. We further demonstrate that the hole accumulation layer in exfoliated SnSe transistors exhibits a field effect mobility of up to $250\phantom{\rule{0.16em}{0ex}}{\mathrm{cm}}^{2}/\mathrm{V}\phantom{\rule{0.16em}{0ex}}\mathrm{s}$ at $T=1.3\phantom{\rule{0.16em}{0ex}}\mathrm{K}$. SnSe is thus found to be a high-quality quasi-two-dimensional semiconductor ideal for thermoelectric applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.273
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0020.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.004

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.374
Teacher spread0.359 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations55
Published2018
Admission routes2
Has abstractyes

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