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Record W2790278121 · doi:10.1002/cjce.23186

Advanced treatment of phenol by H<sub>2</sub>O<sub>2</sub>/UV/activated carbon coupling: Influence of homogeneous and heterogeneous phase

2018· article· en· W2790278121 on OpenAlexvenueno aff
Alexandre Flouret, Maria Carolina de Almeida, Tatianne Ferreira de Oliveira, Fernando Pereira de Sá

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2018
Typearticle
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsnot available
Fundersnot available
KeywordsHydrogen peroxidePhenolChemistryScavengerAqueous solutionKineticsPhase (matter)Activated carbonPeroxideDegradation (telecommunications)Reaction rate constantCatalysisHomogeneousAqueous two-phase systemRadicalCarbon fibersNuclear chemistryOrganic chemistryMaterials scienceComposite numberThermodynamics

Abstract

fetched live from OpenAlex

Abstract In this work, a heterogeneous catalytic wet peroxide process combining activated carbon (AC) and hydrogen peroxide (H2O2)/ultraviolet radiation was applied for the aqueous‐phase removal of phenol. The influence of the pH and peroxide concentration were determined according to a factorial plan. The kinetic contribution of radical mechanisms ( ) was estimated using a radical scavenger (tert‐butyl alcohol). The degradation kinetics was modelled by a global pseudo‐first‐order kinetic model based on the sum of the effects during the treatment process. The results showed that these two variables significantly affected the percentage removal. The peroxide concentration exerted a positive effect (i.e., as the H2O2 concentration increased, the percentage removal also increased). Additionally, as the pH value increased, the degradation accelerated, and the kinetic constant (khomogeneous) increased from 0.00938 min−1 to 0.02772 min−1. The results obtained in the presence of AC demonstrated the ability of AC to ameliorate the degradation of phenol; for example, was 45.69 % to 41.35 %.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.216
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2018
Admission routes1
Has abstractyes

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