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Record W2790382046 · doi:10.1149/2.0841802jes

Explicit Conversion between Different Equivalent Circuit Models for Electrochemical Impedance Analysis of Lithium-Ion Cells

2018· article· en· W2790382046 on OpenAlexafffund
Sam Buteau, Douglas C. Dahn, J. R. Dahn

Bibliographic record

VenueJournal of The Electrochemical Society · 2018
Typearticle
Languageen
FieldEngineering
TopicAdvanced Battery Technologies Research
Canadian institutionsUniversity of Prince Edward IslandDalhousie University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsEquivalent circuitElectronic circuitElectrical impedanceDielectric spectroscopyResistorElectronic engineeringConstant phase elementHigh impedanceRC circuitCapacitorComputer scienceElectrical engineeringMaterials scienceChemistryElectrochemistryVoltageEngineeringElectrodePhysical chemistry

Abstract

fetched live from OpenAlex

Despite the accuracy and non-intrusive nature of Electrochemical Impedance Spectroscopy, the impedance spectra of commercial Lithium-ion cells are notoriously hard to interpret. Consequently, the literature is filled with various equivalent circuit models, which differ greatly in their physical significance, but which produce very similar impedance spectra. In this paper, explicit formulas are given to convert between various equivalent circuits made of resistors and capacitors of the sort discussed in the literature. Furthermore, all these formulas have been implemented in a Python program, in the hope that studies done assuming one circuit might be compared to studies done with a different circuit, for instance. This paper considers cases where two different circuits can produce two impedance spectra which are identical. For instance, explicit conversions are given between Ladder circuits, Voight circuits, and Maxwell circuits for various time constants. This gives a conceptual foundation to explore the more difficult case of circuits producing impedance spectra which are similar to each other (e.g. within 5%).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.004
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.006
Threshold uncertainty score0.020

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.004
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0020.003
Open science0.0020.001
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.0060.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.271
Teacher spread0.247 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2018
Admission routes2
Has abstractyes

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