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Record W2792012239 · doi:10.1080/09593330.2018.1430173

Real-time monitoring of nanoscale TiO <sub>2</sub> concentration by spectrophotometry: implications of agglomeration due to natural organic matter and multivalent ions

2018· article· en· W2792012239 on OpenAlexafffund
Andrew B. Holmes, Frank Gu

Bibliographic record

VenueEnvironmental Technology · 2018
Typearticle
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsSpectrophotometryWastewaterSlurryEnvironmental chemistryInductively coupled plasma mass spectrometryNatural organic matterOrganic matterSewage treatmentEnvironmental scienceInductively coupled plasmaChemistryEnvironmental monitoringMass spectrometryEnvironmental engineeringWater treatmentChromatographyPlasma

Abstract

fetched live from OpenAlex

The study of the environmental fate of nanoscale TiO2 (n-TiO2) is a major recent research focus which requires a rapid and accurate on-site concentration determination method. Inductively coupled plasma mass spectroscopy (ICP-MS) has been the most widely used method for determining the concentration of n-TiO2 in environmental samples; however, poses many challenges, such as hazardous hydrofluoric acid pre-treatment and clear limitations in mobile on-site measurement and monitoring. This study demonstrates that industrial wastewater containing natural organic matter (NOM) can present a major challenge to the analysis of n-TiO2 by ICP-MS, and introduces a spectrophotometry technique that can be used as an alternative. The results suggest that spectrophotometry methods can be more accurate than slurry nebulization ICP-MS for measuring the concentrations of n-TiO2 in wastewater containing NOM under low salt conditions. Furthermore, this study demonstrates the use of a portable flow-through spectrophotometer for use in applications of wastewater treatment and environmental monitoring with real-time feedback of n-TiO2 concentrations. The ability to detect and monitor n-TiO2 will greatly assist in improving the understanding of hazards and risks that emerging nanomaterials pose to the environment and the public health.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.630

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.234
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2018
Admission routes2
Has abstractyes

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