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Record W2795071326 · doi:10.1021/acs.est.7b06608

Exploring Conditions for Ultrafine Particle Formation from Oxidation of Cigarette Smoke in Indoor Environments

2018· article· en· W2795071326 on OpenAlexafffund
Chen Wang, Douglas B. Collins, Rachel F. Hems, Nadine Borduas‐Dedekind, María Antiñolo, Jonathan P. D. Abbatt

Bibliographic record

VenueEnvironmental Science & Technology · 2018
Typearticle
Languageen
FieldEnvironmental Science
TopicAir Quality and Health Impacts
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaUniversidad de Castilla-La ManchaAlfred P. Sloan Foundation
KeywordsSmokeUltrafine particleCigarette smokeParticle (ecology)Environmental scienceEnvironmental chemistryChemistryWaste managementEnvironmental healthChemical engineeringEngineeringGeology

Abstract

fetched live from OpenAlex

Cigarette smoke is an important source of particles and gases in the indoor environment. In this work, aging of side-stream cigarette smoke was studied in an environmental chamber via exposure to ozone (O 3 ), hydroxyl radicals (OH) and indoor fluorescent lights. Aerosol mass concentrations increased by 13–18% upon exposure to 15 ppb O 3 and by 8–42% upon exposure to 0.45 ppt OH. Ultrafine particle (UFP) formation was observed during all ozone experiments, regardless of the primary smoke aerosol concentration (185–1950 μg m –3 ). During OH oxidation, however, UFP formed only when the primary particle concentration was relatively low (<130 μg m –3 ) and the OH concentration was high (∼1.1 × 10 7 molecules cm –3 ). Online aerosol composition measurements show that oxygen- and nitrogen- containing species were formed during oxidation. Gas phase oxidation of NO to NO 2 occurred during fluorescent light exposure, but neither primary particle growth nor UFP formation were observed. Overall, exposure of cigarette smoke to ozone will likely lead to UFP formation in indoor environments. On the other hand, UPF formation via OH oxidation will only occur when OH concentrations are high (∼10 7 molecules cm –3 ), and is therefore less likely to have an impact on indoor aerosol associated with cigarette smoke.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.079
GPT teacher head0.302
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2018
Admission routes2
Has abstractyes

Explore more

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