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Record W2799111283 · doi:10.1103/physrevb.98.214422

Origin of magnetic excitation gap in double perovskite <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Sr</mml:mi><mml:mn>2</mml:mn></mml:msub><mml:msub><mml:mi>FeOsO</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>

2018· article· lv· W2799111283 on OpenAlexafffund
A. E. Taylor, Ryan Morrow, M. D. Lumsden, Stuart Calder, M. H. Upton, А. И. Колесников, M. B. Stone, R. S. Fishman, Arun Paramekanti, Patrick M. Woodward, A. D. Christianson

Bibliographic record

VenuePhysical review. B./Physical review. B · 2018
Typearticle
Languagelv
FieldPhysics and Astronomy
TopicAdvanced Condensed Matter Physics
Canadian institutionsUniversity of TorontoCanadian Institute for Advanced Research
FundersArgonne National LaboratoryBasic Energy SciencesNatural Sciences and Engineering Research Council of CanadaRussian Science FoundationOak Ridge National LaboratoryAlexander von Humboldt-StiftungU.S. Department of EnergyDivision of Materials ResearchOffice of ScienceNational Science Foundation
KeywordsInelastic neutron scatteringAntiferromagnetismMultipletPerovskite (structure)PhysicsResonant inelastic X-ray scatteringExcited stateCondensed matter physicsGround stateCrystallographyNeutron scatteringScatteringAtomic physicsChemistrySpectral lineOpticsQuantum mechanics

Abstract

fetched live from OpenAlex

${\mathrm{Sr}}_{2}{\mathrm{FeOsO}}_{6}$ is an insulating double perovskite compound which undergoes antiferromagnetic transitions at 140 (${T}_{\text{N1}}$) and 67 K (${T}_{\text{N2}}$). To study the underlying electronic and magnetic interactions giving rise to this behavior we have performed inelastic neutron scattering (INS) and resonant inelastic x-ray scattering (RIXS) experiments on polycrystalline samples of ${\mathrm{Sr}}_{2}{\mathrm{FeOsO}}_{6}$. The INS data reveal that the spectrum of spin excitations remains ungapped below ${T}_{\text{N1}}$, however below ${T}_{\text{N2}}$ a gap of 6.8 meV develops. The RIXS data reveals splitting of the ${T}_{2g}$ multiplet consistent with that seen in other $5{d}^{3}$ osmium based double perovskites. Together these results suggest that spin-orbit coupling is important for ground state selection in $3d\text{\ensuremath{-}}5{d}^{3}$ double perovskite materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.924
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0020.003
Meta-epidemiology (broad)0.0010.004
Bibliometrics0.0000.003
Science and technology studies0.0010.003
Scholarly communication0.0010.002
Open science0.0030.002
Research integrity0.0010.003
Insufficient payload (model declined to judge)0.2000.008

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.295
Teacher spread0.272 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2018
Admission routes2
Has abstractyes

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