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Record W2805715982 · doi:10.1002/marc.201800214

Wurster‐Type Anthanthrene Polyradicaloid Cations

2018· article· en· W2805715982 on OpenAlexaff
Maude Desroches, Jean‐François Morin

Bibliographic record

VenueMacromolecular Rapid Communications · 2018
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsUniversité Laval
Fundersnot available
KeywordsCationic polymerizationSteric effectsDiphenylaminePolymerElectron paramagnetic resonanceMacromoleculePlanarity testingPolymer chemistryRadicalChemistryPhotochemistryAbsorption (acoustics)Materials scienceCrystallographyStereochemistryOrganic chemistryNuclear magnetic resonance

Abstract

fetched live from OpenAlex

4,10-dibromoanthanthrone, a highly robust building block, is used to synthesize a bis(triarylamine) polymer. The polymer can be oxidized twice to form a polycationic macromolecule showing magnetic properties by electron paramagnetic resonance spectroscopy. In its dicationic state, the presence of isolated radicals is possible because of the interrupted conjugation between the diphenylamine with the anthanthrone core. The high steric hindrance prevents the planarity of the adjacent groups resulting in a polyradical cationic polymer. The oxidized polymer has a strong absorption in the near-infrared region along with reversible redox stages.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.233
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0000.000
Open science0.0020.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.039
GPT teacher head0.312
Teacher spread0.273 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2018
Admission routes1
Has abstractyes

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