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In Situ Remediation Method for Enhanced Sorption of Perfluoro-Alkyl Substances onto Ottawa Sand

2018· article· en· W2826231799 on OpenAlexaboutno aff
Yousof H. Aly, Chen Liu, Daniel P. McInnis, Bonnie A. Lyon, James Hatton, Michael McCarty, William A. Arnold, Kurt D. Pennell, Matt F. Simcik

Bibliographic record

VenueJournal of Environmental Engineering · 2018
Typearticle
Languageen
FieldEnvironmental Science
TopicPer- and polyfluoroalkyl substances research
Canadian institutionsnot available
Fundersnot available
KeywordsPerfluorooctanoic acidSorptionEnvironmental remediationAdsorptionChemistryEnvironmental chemistryAlkylGroundwater remediationGroundwaterChlorideIn situContaminationOrganic chemistryGeologyGeotechnical engineering

Abstract

fetched live from OpenAlex

Perfluoro-alkyl substances (PFAS) have drawn increased concern in recent years. Due to resistance to many remediation methods and potential for long-range transport, there is need for continued in situ remediation technique development. One such method is enhanced sorption onto aquifer material, thereby sequestering a plume and preventing long-range migration. Batch tests and column studies were carried out to evaluate the ability of polydiallyldimethylammonium chloride (PDM) and polyamine (PA) to enhance the adsorption of six PFAS onto Ottawa sand. At a dosage of 2,000 mg/L of either PDM or PA, results show increases of adsorption of the tested PFAS in all batches by factors of 3.6–45. Column studies showed retention capacity increasing up to six times for perfluorooctanoic acid (PFOA) and 10 times for perfluorooctane sulfonic acid (PFOS). Normalizing partitioning coefficients from batch tests to fraction of organic carbon suggest that an interaction other than PFAS associating with organic matter may be the main driving force behind sorption enhancement. These results suggest that this method shows promise for in situ remediation of PFAS-contaminated groundwater.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.043
Threshold uncertainty score0.085

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.264
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations49
Published2018
Admission routes1
Has abstractyes

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Same venueJournal of Environmental EngineeringSame topicPer- and polyfluoroalkyl substances researchFrench-language works237,207