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Record W2884508853 · doi:10.1039/c8an01117f

Development of an electrochemical surface-enhanced Raman spectroscopy (EC-SERS) fabric-based plasmonic sensor for point-of-care diagnostics

2018· article· en· W2884508853 on OpenAlex
Shruti D. Bindesri, Dalal S. Alhatab, Christa L. Brosseau

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueThe Analyst · 2018
Typearticle
Languageen
FieldMaterials Science
TopicGold and Silver Nanoparticles Synthesis and Applications
Canadian institutionsSaint Mary's University
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanada Foundation for InnovationNova Scotia Research Innovation TrustMinistry of Higher Education and Scientific Research
KeywordsWearable computerMaterials scienceNanotechnologyElectrodeSurface-enhanced Raman spectroscopyRaman spectroscopyPoint of careBiomedical engineeringOptoelectronicsComputer scienceRaman scatteringChemistryOpticsMedicineEmbedded system

Abstract

fetched live from OpenAlex

Early disease diagnosis is crucial for timely and effective healthcare monitoring and treatment. Demand for modern point-of-care (POC) technologies has increased during the past decade. Continuous monitoring of patient health status can be achieved through wearable sensors which can be incorporated into clothing and other wearables. While electronic textiles that monitor physical parameters (heart rate, blood pressure, etc.) are increasingly commonplace, smart textiles capable of monitoring chemical biomarkers are much less common. In this work, a conductive plasmonic electrochemical sensor was developed from a cotton blend fabric modified with silver nanoparticles and conductive inks. para-Aminothiophenol (pATP) was used as an initial probe molecule to evaluate the performance of the fabric-based electrode for electrochemical surface-enhanced Raman spectroscopic (EC-SERS) measurements. Further investigation was then carried out to detect levofloxacin, a commonly prescribed antibiotic, in both 0.1 M NaF and synthetic urine as supporting electrolyte. It was found that the fabric-based electrode provided excellent EC-SERS signals, comparable to commercial screen-printed electrodes, allowing for rapid detection of levofloxacin at clinically relevant concentrations. To the best of our knowledge, this is the first time a fabric-based electrode has been reported for EC-SERS investigations, highlighting a promising platform for wearable point-of-care sensors.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.036
Threshold uncertainty score0.315

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.271
Teacher spread0.257 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it