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Record W2888361599 · doi:10.1021/acssuschemeng.8b01972

Enhanced High-Solids Fed-Batch Enzymatic Hydrolysis of Sugar Cane Bagasse with Accessory Enzymes and Additives at Low Cellulase Loading

2018· article· en· W2888361599 on OpenAlex
Marie Rose Mukasekuru, Jinguang Hu, Xiaoqin Zhao, Fubao Sun, Kaneza Pascal, Hongyan Ren, Junhua Zhang

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2018
Typearticle
Languageen
FieldEngineering
TopicBiofuel production and bioconversion
Canadian institutionsUniversity of British Columbia
FundersChangjiang Scholar Program of Chinese Ministry of EducationMinistry of FinanceNatural Science Foundation of Jiangsu ProvinceState Administration of Foreign Experts AffairsGovernment of Jiangsu ProvinceChina Postdoctoral Science FoundationMinistry of Education of the People's Republic of ChinaNational Natural Science Foundation of China
KeywordsCellulaseEnzymatic hydrolysisHydrolysisChemistryBagasseCelluloseSubstrate (aquarium)Lignocellulosic biomassXylanaseBiorefineryChromatographyOrganic chemistryEnzymePulp and paper industryRaw material

Abstract

fetched live from OpenAlex

High cellulase loading is still a major impediment in the production of fermentative sugars from high-solids enzymatic hydrolysis of lignocellulosic substrates in the enzyme-based “biorefinery” industry. This study attempted a high-solids (20%) enzymatic hydrolysis of lignocellulosic substrate at a very low cellulase loading with mixed use of additives and accessory enzymes by fed-batch mode. To avoid the high initial biomass viscosity, the high-solids enzymatic hydrolysis of lignocellulosic substrates was initiated with a solids content of 8%. Thereafter, 4% of the additional substrates were consecutively fed into the hydrolysis system after 6, 12, and 18 h to reach a final solids content of 20%. Some additive mixtures (40 mg/g substrateTween 80 + 10 mg/g substrate tea saponin +20 mg/g substrate BSA) were observed to enable this fed-batch hydrolysis to increase 30% of the glucose yield after the 48 h. The combination of these additives and accessory enzymes (2.4 mg/g substrate xylanase and 1 mg/g substrate AA9) in the high-solids hydrolysis system further boosted the sugar release. This allowed us to achieve an industrially relevant sugar yield (83% cellulose and 90% xylan hydrolysis) and fermentable sugar titer (∼160 g/L) after 72 h, with a low cellulase enzyme loading (3 FPU/g substrate). Our results indicate that the fed-batch substrate addition process is a favorable model for high-solids enzymatic hydrolysis of lignocellulosic substrates. Moreover, the synergism between the additives and accessory enzymes can greatly boost the high-solids enzymatic hydrolysis of lignocellulosic substrates.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.168
Teacher spread0.166 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it