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Record W2900469313 · doi:10.1073/pnas.1809187115

Elastic and Li-ion–percolating hybrid membrane stabilizes Li metal plating

2018· article· en· W2900469313 on OpenAlexafffund
Quanquan Pang, Laidong Zhou, Linda F. Nazar

Bibliographic record

VenueProceedings of the National Academy of Sciences · 2018
Typearticle
Languageen
FieldEngineering
TopicAdvanced Battery Materials and Technologies
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of CanadaGovernment of Canada
KeywordsElectrolyteMaterials scienceMembraneElectrodeElectrochemistryMetalPlating (geology)Chemical engineeringBattery (electricity)Stripping (fiber)Composite materialNanotechnologyChemistryMetallurgy

Abstract

fetched live from OpenAlex

Significance Lithium metal batteries are capable of revolutionizing the battery marketplace for electrical vehicles. They are, however, plagued by the reactive Li metal–electrolyte interface and growth of Li dendrites on cycling, which pose concerns to both cell performance and safety. We demonstrate that a Li metal negative electrode can be stabilized by a hybrid inorganic/organic membrane that is grown directly onto it. A solid electrolyte phase offers percolated Li + -ion–conducting channels and the infiltration of an elastic polymer endows membrane flexibility to accommodate volume changes. The protected electrode allows Li deposition/stripping with 95.8% efficiency and stable operation of an electrochemical cell for 2,000 cycles. This rationally structured membrane represents an interface engineering approach toward stabilized Li metal electrodes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.038
Threshold uncertainty score0.270

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.264
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations73
Published2018
Admission routes2
Has abstractyes

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