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Record W2900520721 · doi:10.15278/isms.2018.wk10

ROTATIONAL SPECTRA AND GEOMETRIES OF FOUR CONFORMERS OF ISOLATED UROCANIC ACID; AND OF A COMPLEX OF UROCANIC ACID WITH WATER

2018· article· en· W2900520721 on OpenAlexaboutno aff
Nick Walker, Eva Gougoula, Chris Medcraft, Graham A. Cooper

Bibliographic record

VenueProceedings of the 73rd International Symposium on Molecular Spectroscopy · 2018
Typearticle
Languageen
FieldChemistry
TopicChemical Thermodynamics and Molecular Structure
Canadian institutionsnot available
Fundersnot available
KeywordsUrocanic acidConformational isomerismSpectral lineChemistryStereochemistryBiochemistryOrganic chemistryPhysicsMoleculeEnzymeAstronomy

Abstract

fetched live from OpenAlex

The Montreal Protocol has banned the production of major ozone depleting substances such as chlorofluorocarbons (CFCs) to protect the Earth’s ozone layer. These chlorinated compounds eventually form a large reservoir of \\chem{HCl} in the upper atmosphere. Therefore, the success of the Montreal Protocol can be determined by measuring the stratospheric \\chem{HCl} abundance. The Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) measures infrared solar occultation spectra of the Earth’s atmosphere from which altitude profiles of \\chem{HCl} volume mixing ratios (VMRs) are determined. The stratospheric \\chem{HCl} VMR time series has a linear trend of -4.9$\\pm{0.4} $\\% per decade for 2004-2017, highlighting the continuing success of the Montreal Protocol. The emission of hydrofluorocarbons (HFCs) has increased in order to replace the CFCs since they are not restricted by the Montreal Protocol. As a result, the atmospheric abundance of HFCs are rapidly increasing. Even though these HFCs do not contribute to the depletion of the ozone layer, they are powerful greenhouse gases with large global warming potentials. In 2016, the Kigali Amendment to the Montreal Protocol was introduced in order to phaseout long-lived HFCs. The VMRs of the two most abundant HFCs in the atmosphere, \\chem{HFC-134a} and \\chem{CHF_3}, are also measured by the ACE-FTS. These measurements will be useful for monitoring the Kigali Amendment to the Montreal Protocol. The ACE observations and trends for atmospheric \\chem{HCl}, \\chem{HFC-134a} and \\chem{CHF_3} will be presented.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.571

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.215
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2018
Admission routes1
Has abstractyes

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