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Record W2900945670 · doi:10.1111/maps.13580

UV laser‐induced fluorescence spectroscopy as a non‐destructive technique for mineral and organic detection in carbonaceous chondrites

2020· article· en· W2900945670 on OpenAlexafffundabout
Elizabeth A. Lymer, M. G. Daly, K. T. Tait, V. E. Di Cecco, E.A. Lalla

Bibliographic record

VenueMeteoritics and Planetary Science · 2020
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAstro and Planetary Science
Canadian institutionsRoyal Ontario MuseumYork University
FundersNatural Sciences and Engineering Research Council of CanadaCanadian Space Agency
KeywordsMurchison meteoriteRaman spectroscopyChondriteSpectroscopyMineralFluorescenceFluorescence spectroscopyAnalytical Chemistry (journal)Carbonaceous chondriteLaser-induced breakdown spectroscopyLaser-induced fluorescenceMeteoriteChemistryMaterials scienceMineralogyAstrobiologyOpticsEnvironmental chemistryPhysicsAstronomy

Abstract

fetched live from OpenAlex

Abstract Here, we discuss the merits of non‐destructive UV laser‐induced fluorescence spectroscopy (LIF) as a flight or laboratory instrument to analyze organic and mineral material in samples on or returned from carbon‐rich asteroids such as (101955) Bennu by NASA’s OSIRIS‐REx mission. LIF is a unique instrument that is non‐destructive while acquiring data, and allows for no sample preparation, crushing, or cutting. This method provides spectral data indicative of specific minerals and organics in less time than Raman spectroscopy, and can be set up to produce 2‐D raster images of areas of interest. Furthermore, if an LIF system is set up with a gated CCD camera, time‐resolved fluorescence spectroscopy can be performed, providing a unique identification tool for organic and mineral contents using fluorescence decay over several nanoseconds. This technique was used to analyze millimeter‐sized chondrules and calcium‐aluminum‐rich inclusions on four carbonaceous chondrite samples provided by the Royal Ontario Museum: Murchison (CM2), Allende (CV3), NWA 11554 (CV3), and NWA 12796 (CK3). The LIF 2‐D maps, point spectra, and time‐resolved fluorescence data and mineral identifications using LIF were compared to that of well‐known techniques such as Raman spectroscopy and SEM/EDS.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.216
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2020
Admission routes3
Has abstractyes

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