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Record W2901490983 · doi:10.1002/cjce.23339

Evolution of electronic conductivity in a Ni/YSZ electrode fabricated by electrophoretic deposition

2018· article· en· W2901490983 on OpenAlexafffundvenue
Saeid Amiri, Robert E. Hayes, Partha Sarkar

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2018
Typearticle
Languageen
FieldMaterials Science
TopicAdvancements in Solid Oxide Fuel Cells
Canadian institutionsAlberta InnovatesUniversity of Alberta
FundersAlberta Innovates - Technology Futures
KeywordsMaterials scienceElectrophoretic depositionYttria-stabilized zirconiaAnodeThermal conductivityConductivityDeposition (geology)ElectrodeOxideSolid oxide fuel cellBreakageFabricationAnalytical Chemistry (journal)Composite materialChemical engineeringMetallurgyChemistryCubic zirconiaCeramic

Abstract

fetched live from OpenAlex

Abstract The conductivity of a tubular micro solid oxide fuel cell (TμSOFC) anode is measured in‐situ. The Ni/YSZ composite anode was fabricated using the electrophoretic deposition (EPD) technique. The four‐probe method is used to measure the conductivity of several samples simultaneously under a reducing atmosphere during several cycles of heating, ∼100 h dwelling and cooling periods. Special attention is paid to maintaining similar fabrication and thermal histories among the samples. Despite all this, the measured conductivities show substantial variation and degradation from sample to sample and from one thermal cycle to the next. The most variations occur during the reduction of the cell, with significant oscillations in the measurements. Sample conductivities exhibit step‐like changes during the cooling and heat‐up cycles. A theory based on thermal expansion induced Ni particles connection formation and breakage within the YSZ backbone is proposed. Sample electron microscope micrographs are presented showing island‐like segregated Ni particles within a continuous YSZ structure. Eliminating such effects not only will reduce the cell performance variability but will also increase the peak power by 60 %, according to our simulation results.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.199
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2018
Admission routes3
Has abstractyes

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Same venueThe Canadian Journal of Chemical EngineeringSame topicAdvancements in Solid Oxide Fuel CellsFrench-language works237,207