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Record W2911998861 · doi:10.1107/s0108767318098537

Effect of addition of lanthanum on the hydrogen storage properties of TiFe alloy

2018· article· en· W2911998861 on OpenAlexaff
M. Meraj Alam, Pratibha Sharma, Jacques Huot

Bibliographic record

VenueActa Crystallographica Section A Foundations and Advances · 2018
Typearticle
Languageen
FieldMaterials Science
TopicHydrogen Storage and Materials
Canadian institutionsUniversité du Québec à Trois-Rivières
Fundersnot available
KeywordsLanthanumHydrogen storageAlloyMaterials scienceHydrogenMetallurgyInorganic chemistryChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

TiFe is one of the good candidates for the solid-state hydrogen storage.Despite having fast kinetics and fairly good capacity, it's first hydrogenation is difficult.In this study, we investigated the effect of addition of lanthanum on the hydrogen storage properties of TiFe alloy.As the melting point of lanthanum is much lower than the ones of the other two elements, synthesis by casting was impossible.Instead ball milling was used to synthesize the compound.It was found that the TiFe alloy is formed after 5 hours of milling.The hydrogen storage properties were measured at room temperature and at a pressure of up to 40 bars on a home-made Sievert's apparatus.For the first hydrogenation, the alloy absorbed 1 wt.% of hydrogen in less than 5 minutes.But, the first de-hydrogenation showed a reduced capacity from 1 wt% to 0.65 wt% i.e., a reduction of 0.35 wt%.Further hydrogenation and dehydrogenation shows no further loss in capacity.To understand the loss in capacity, the X-ray diffraction of fully hydrogenated and fully dehydrogenated samples were performed.But from these diffraction patterns a secondary phase was observed.The presence of this secondary phase may explain the loss of capacity.Possible crystal structure of this phase will be discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.250
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations1
Published2018
Admission routes1
Has abstractyes

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Same venueActa Crystallographica Section A Foundations and AdvancesSame topicHydrogen Storage and MaterialsFrench-language works237,207