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Record W2911998861 · doi:10.1107/s0108767318098537

Effect of addition of lanthanum on the hydrogen storage properties of TiFe alloy

2018· article· en· W2911998861 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueActa Crystallographica Section A Foundations and Advances · 2018
Typearticle
Languageen
FieldMaterials Science
TopicHydrogen Storage and Materials
Canadian institutionsUniversité du Québec à Trois-Rivières
Fundersnot available
KeywordsLanthanumHydrogen storageAlloyMaterials scienceHydrogenMetallurgyInorganic chemistryChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

TiFe is one of the good candidates for the solid-state hydrogen storage. Despite having fast kinetics and fairly good capacity, it's first hydrogenation is difficult. In this study, we investigated the effect of addition of lanthanum on the hydrogen storage properties of TiFe alloy. As the melting point of lanthanum is much lower than the ones of the other two elements, synthesis by casting was impossible. Instead ball milling was used to synthesize the compound. It was found that the TiFe alloy is formed after 5 hours of milling. The hydrogen storage properties were measured at room temperature and at a pressure of up to 40 bars on a home-made Sievert's apparatus. For the first hydrogenation, the alloy absorbed 1 wt.% of hydrogen in less than 5 minutes. But, the first de-hydrogenation showed a reduced capacity from 1 wt% to 0.65 wt% i.e., a reduction of 0.35 wt%. Further hydrogenation and dehydrogenation shows no further loss in capacity. To understand the loss in capacity, the X-ray diffraction of fully hydrogenated and fully dehydrogenated samples were performed. But from these diffraction patterns a secondary phase was observed. The presence of this secondary phase may explain the loss of capacity. Possible crystal structure of this phase will be discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score0.385

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.250
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it